The wide applications of terahertz (THz) wave technology in the ∼1–3 THz range has resulted in a surge in the demand for the performance improvement of THz wave detection technique. In this study, a frequency tunable, highly sensitive frequency upconversion detection based on a 2-(3-(4-hydroxystyryl)-5,5-dime-thylcyclohex-2-enylidene) malononitrile (OH1) crystal at room temperature is demonstrated. Moreover, to effectively increase the signal-to-noise ratio in the low frequency range, a beam isolation enhancer is proposed and its effect is verified. The minimum detectable THz pulse energy reaches about 100 aJ at 1.9 THz. The frequency tuning ranging from 1 to 3 THz. Sensitivity comparison with a 4-dimethylamino-N-methyl-4-stilbazolium tosylate (DAST) crystal system shows that OH1 is a more suitable nonlinear crystal in the 1–2.4 THz range.

We demonstrate an all-solid-state widely wavelength-tunable Y b : Y S r 3 ( P O 4 ) 3 (Yb:YSP) laser with high efficiency. The free-running Yb:YSP laser oscillating at multiple wavelengths in the range of 1024–1054 nm is realized with different crystal lengths and output coupler transmittances. The maximum output power of 2.72 W is obtained under the absorption pump power of 7.30 W. The highest slope efficiency is 66.9%, using the crystal of 6.5-mm-length. Simultaneous dual-wavelength operation can be realized as well. Furthermore, the widely wavelength-tunable Yb:YSP laser with a range of more than 60 nm (from 1004 to 1066 nm) is achieved using a birefringent filter. The experimental results indicate that the Yb:YSP crystal can be a promising candidate for ultrafast lasers in the 1 µm region.

A novel disordered crystal Yb:YSr ₃ (PO ₄ ) ₃ is grown by the Czochralski method. Results indicate that it can be a promising candidate for ultrashort pulse generation and tunable broadband solid-state lasers.

Frequency upconversion technology with good performance including high sensitivity, fast response, and room-temperature operation is a promising method for terahertz-wave detection. The sum-frequency conversion and difference-frequency conversion jointly affect the detection ability for upconversion detection using organic crystals as nonlinear media. The concurrence of both processes has been ignored in past studies, which results in discrepancies between theoretical simulations and experimental results. In this paper, four-wave interaction equations involving two nonlinear conversion processes are proposed, and the effect of the sum-frequency process is analyzed in upconversion terahertz-wave detection via a 4-dimethylamino-N-methyl-4-stilbazolium tosylate (DAST) crystal. The ratio of the sum-frequency signal to the difference-frequency signal varies for different terahertz frequencies and crystal thicknesses. Experiments suggest that theoretical simulations are good at predicting physical processes. Under certain conditions, the detection efficiency can be improved by simultaneously utilizing the two signals. The total signal photon number is not sensitive to the crystal thickness. Furthermore, the theoretical exploration of terahertz single-photon detection provides a noteworthy reference for future experiments.

Terahertz spectroscopy systems, which integrate terahertz sources and detectors, have important applications in many fields such as materials science and security checking. Based on highly sensitive frequency up-conversion detection, large dynamic range spectral measurements in a terahertz region are reported. Our system realized the detection sensitivity at a 10 aJ level with a 2-(3-(4-hydroxystyryl)-5,5-dime-thylcyclohex-2-enylidene) malononitrile (OH1) crystal and a dynamic range up to seven orders. Based on this system, we verified the validity of the spectral measurement with tests which were conducted on monohydrate glucose, anhydrous glucose and mixed tablet samples with a thickness of 0.8 mm in 1~3 THz, respectively. Also, a mini coppery elbow tube with an inner diameter of 1 mm was used for the transmission of a terahertz wave to simulate some strip biological tissue samples. By allowing terahertz to transmit through this tube filled with 0.5 g glucose powder, we successfully obtained the absorption spectrum with a minimum transmittance at the absorption peak in the order of 10⁻⁴.