An optimal model was developed for accounting forest carbon stock from synergistic use of optical data from Landsat TM and synthetic aperture radar (SAR) data from COSMO-Skymed (X-band), Radarsat-2 (C-band) and ALOS PALSAR (L-band) sensors over a tropical deciduous heterogeneous forest of India. The best-fit integrated multiple linear regression model had a model accuracy of 83%, r² = 0.96, root mean square error = 10.02 Mg/ha and Willmott’s index of agreement of 0.98. The model further validated using chi-squared and t-test. Results of models for calculating the aboveground biomass (AGB) were converted to C and CO₂ using conversion factors. Average AGB, C and CO₂ were 70.5, 35.26 and 130.89 Mg/ha, respectively. The synergistic use of optical and multi-frequency SAR data enhanced the AGB saturation threshold to about 150 Mg/ha for tropical deciduous mixed forests. Hence, the synergistic use of this data is suggested for large-scale AGB and C estimations for tropical forests. Optical remote sensing sensors are extensively used due to greater data availability despite their poor sensitivity toward forest parameters. In contrast, SAR signals are highly sensitive toward forest biophysical and structural parameters, providing a better alternative. This unique integrated approach provides valuable information regarding the spatial distribution and quantification of forest biomass and carbon.