Neutrinoless double beta decay ($0\nu \beta \beta$) provides a way to probe physics beyond the Standard Model of particle physics. The upcoming nEXO experiment will search for $0\nu \beta \beta$ decay in ¹³⁶Xe with a projected half-life sensitivity exceeding ${10}^{28}$ years at the 90% confidence level using a liquid xenon (LXe) Time Projection Chamber (TPC) filled with 5 tonnes of Xe enriched to ∼90% in the $\beta \beta$-decaying isotope ¹³⁶Xe. In parallel, a potential future upgrade to nEXO is being investigated with the aim to further suppress radioactive backgrounds and to confirm $\beta \beta$-decay events. This technique, known as Ba-tagging, comprises extracting and identifying the $\beta \beta$-decay daughter ¹³⁶Ba ion. One tagging approach being pursued involves extracting a small volume of LXe in the vicinity of a potential $\beta \beta$-decay using a capillary tube and facilitating a liquid-to-gas phase transition by heating the capillary exit. The Ba ion is then separated from the accompanying Xe gas using a radio-frequency (RF) carpet and RF funnel, conclusively identifying the ion as ¹³⁶Ba via laser-fluorescence spectroscopy and mass spectrometry. Simultaneously, an accelerator-driven Ba ion source is being developed to validate and optimize this technique. The motivation for the project, the development of the different aspects, along with the current status and results, are discussed here.

nEXO is a proposed experiment that will search for neutrinoless double-beta decay (0$νββ$) in 5-tonnes of liquid xenon (LXe), isotopically enriched in $^{136}$Xe. A technique called Ba-tagging is being developed as a potential future upgrade for nEXO to detect the $^{136}$Xe double-beta decay daughter isotope, $^{136}$Ba. An efficient Ba-tagging technique has the potential to boost nEXO's 0$νββ$ sensitivity by essentially suppressing non-double-beta decay background events. A conceptual approach for the extraction from the detector volume, trapping, and identification of a single Ba ion from 5 tonnes of LXe is presented, along with initial results from the commissioning of one of its subsystems, a quadrupole mass filter.

The next generation of rare-event search experiments in nuclear and particle physics demand structural materials combining exceptional mechanical strength with ultra-low levels of radioactive contamination. This study evaluates chemical vapor deposition (CVD) nickel as a candidate structural material for such applications. Manufacturer-supplied CVD Ni grown on aluminum substrates underwent tensile testing before and after welding alongside standard Ni samples. CVD Ni exhibited a planar tensile strength of ~600 MPa, significantly surpassing standard nickel. However, welding and heat treatment were found to reduce the tensile strength to levels comparable to standard Ni, with observed porosity in the welds likely contributing to this reduction. Material assay via inductively coupled plasma mass spectrometry (ICP-MS) employing isotope-dilution produced measured bulk concentration of 232-Th, 238-U, and nat-K at the levels of ~70 ppq, <100 ppq, and ~900 ppt, respectively, which is the lowest reported in nickel. Surface-etch profiling uncovered higher concentrations of these contaminants extending ~10 micrometer beneath the surface, likely associated with the aluminum growth substrate. The results reported are compared to the one other well documented usage of CVD Ni in a low radioactive background physics research experiment and a discussion is provided on how the currently reported results may arise from changes in CVD fabrication or testing process. These results establish CVD Ni as a promising low-radioactivity structural material, while outlining the need for further development in welding and surface cleaning techniques to fully realize its potential in large-scale, low radioactive background rare-event search experiments.