We propose an efficient approach for actively controlling the Rabi oscillations in nanophotonic emitter-cavity analogs based on the presence of an element with optical gain. Inspired by recent developments in parity-time ($\mathcal{PT}$)-symmetry photonics, we show that nano- or microcavities where intrinsic losses are partially or fully compensated by an externally controllable amount of gain offer unique capabilities for manipulating the dynamics of extended (collective) excitonic emitter systems. In particular, we discuss how one can drastically modify the dynamics of the system, increase the overall occupation numbers, enhance the longevity of the Rabi oscillations, and even decelerate them to the point where their experimental observation becomes less challenging. Furthermore, we show that there is a specific gain value that leads to an exceptional point, where both the emitter and cavity occupation oscillate practically in phase, with occupation numbers that can significantly exceed unity. By revisiting a recently introduced Rabi-visibility measure, we provide robust guidelines for quantifying the coupling strength and achieving strong-coupling with adaptable Rabi frequency via loss compensation.

Single-molecule fluorescence spectroscopy offers unique capabilities for the low-concentration sensing and probing of molecular dynmics. However, employing such a methodology for versatile sensing and diagnostics under point-of-care demands device miniaturization to lab-on-a-chip size. In this study, we numerically design metalenses with high numerical aperture (NA = 1.1), which are composed of silicon nitride nanostructures deposited on a waveguide and can selectively focus guided light into an aqueous solution at two wavelengths of interest in the spectral range of 500–780 nm. Despite the severe chromatic focal shift in the lateral directions owing to the wavelength-dependent propagation constant in a waveguide, segmented on-chip metalenses provide perfectly overlapping focal volumes that meet the requirements for epi-fluorescence light collection. We demonstrate that the molecule detection efficiencies of metalenses designed for the excitation and emission wavelengths of ATTO 490LS, Alexa 555, and APC-Cy7 tandem fluorophores are sufficient to collect several thousand photons per second per molecule at modest excitation rate constants. Such sensitivity provides reliable diffusion fluorescence correlation spectroscopy analysis of single molecules on a chip to extract their concentration and diffusion properties in the nanomolar range. Achromatic on-chip metalenses open new avenues for developing ultra-compact and sensitive devices for precision medicine and environmental monitoring.

Mie voids have been recently demonstrated as a promising nanophotonic platform for light manipulation and optical sensing. Moreover, the detection volumes of Mie void cavities exceed those of optical nanoantennas, making them appropriate for low-concentration single-molecule fluorescence biosensing. However, the fluorescence enhancement quantification of diffusing molecules in such optical antenna systems has not been addressed. Here, we explore Mie void ability to enhance the single-molecule fluorescence of diffusing fluorophores AF647 with the help of fluorescence correlation spectroscopy. The optimized structure confines 635 nm laser light within a well-defined excitation volume in the Mie void and provides the excitation intensity enhancement. We monitor the reduction in the number of molecules, signifying the detection volume reduction in the Mie void and an increase in single-molecule brightness up to 2.8 times. However, we reveal that the observed fluorescence enhancement appears limited owing to the azimuthally symmetric emission direction away from the optical axis when the molecules diffuse in the vicinity of the Mie void entrance. Altogether, this study demonstrates exploration of Mie void-based nanoantenna potential for single-molecule fluorescence spectroscopy applications.

It was recently demonstrated in the experiments [1,2] that the internal photoemission efficiency can reach several tens of percents because of “coherent” or, “surface” photoemission. In present work we provide theoretical description of this effect assuming the surface photoemissionin the structureconsisting ofthe Schottky-barrier metal-semiconductor interface with the Quantum Well (QW) inside. We take into account the difference of dielectric permittivities for the metal and the semiconductor which strongly affects the photoemission efficiency. We show that QW inside the Schottky-barrier can lead to (a) lowering the threshold energy of the photoemission due to resonance tunneling of electrons through the intermediate quasi-level of energy in QW; (b) the photoemission efficiency can be increased by several orders of magnitude.

We analyze the emergence of unphysical superluminal group velocities in Su-Schrieffer-Heeger (SSH) parity-time ($\mathcal{PT}$) symmetric chains, and explore the origins of such a behavior. By comparing the band structure of an infinite loss-gain SSH chain with that of a continuous realization—a one-dimensional Bragg stack governed by the Helmholtz equation—we first exclude insufficient coupling consideration in the tight-binding description as the cause of group-velocity divergence. We then focus on material dispersion, and show that indeed, restoring causality in the description of both the lossy and the gain components resolves the problem and recovers finite group velocities, whose real part can only exceed the speed of light in vacuum when accompanied by a significant imaginary part. Our analysis introduces thus the required practical limits in the performance of common $\mathcal{PT}$-symmetric systems.