In this study, jute/polyester composites were fabricated. To improve the adhesion between jute fabric and polyester alkali-treated jute fabrics were treated with γ-methacryloxypropyltrimethoxysilane (γ-MPS). The effect of silane concentrations (0.1%, 0.3%, and 0.5%) on tensile properties, flexural properties, and interlaminar shear strength was investigated. Once jute fabrics were treated with 0.1% and 0.3% silane concentrations, the tensile properties of silane-treated jute polyester composites increased. However, when 0.5% γ-MPS was used in silane treatment, the tensile properties of jute/polyester composites decreased. 0.3% silane-treated jute/polyester composites exhibited superior improvements in terms of the flexure properties among the fabricated composites. Interlaminar shear strength measurements showed that best adhesion was provided by using 0.3% silane-treated jute/polyester composites. Good adhesion between silane-treated jute fabric and polyester was also confirmed by scanning electron microscope observations.