Laboratory for Nano and Micro Mechanics of Materials, Department of Mechanical Engineering Technion, Israel Institute of Technology, Haifa 32000, Israel
Dr. Doron Shilo
Laboratory for Nano and Micro Mechanics of Materials, Department of Mechanical Engineering Technion, Israel Institute of Technology, Haifa 32000, Israel
We apply photoluminescence, photoluminescence excitation, and time-resolved optical spectroscopy for studying a set of periodic structures, which were characterized by high-resolution x-ray diffraction including x-ray mapping in reciprocal space. We found that the energy differences between the absorption edge and the photoluminescence peak (Stokes shift), and the photoluminescence decay time drastically increase with the layer thickness. The decay time strongly increases with the sample temperature. We were able to quite accurately determine the radiative and nonradiative decay times of excitons in these structures by measuring the temperature dependence of the decay times, the integrated photoluminescence intensities, and the photoluminescence intensities immediately after the picosecond excitation pulse. The intrinsic radiative lifetimes, which are inversely proportional to the exciton oscillator strengths, were then calculated from the temperature dependence of the radiative lifetimes. These experimental findings are analyzed using an eight-band model, which quantitatively explains both the Stokes shifts and the intrinsic radiative lifetimes. Their strong dependence on the quantum well width is due to a large (∼1 MV/cm) lattice-mismatch strain-induced piezoelectric field along the growth axis.
X-ray topographs under acoustic wave excitation were taken from LiNbO3-based surface acoustic wave devices with He-implanted waveguide layers, using monochromatized synchrotron radiation from the European Synchrotron Radiation Facility (ESRF), Grenoble. Measurements were performed in the stroboscopic mode, i.e., by synchronizing the electron bunch frequency with the resonant frequency of the acoustic wave excitation in the 300 MHz range. These x-ray diffraction images showed plane acoustic wave propagation through the LiNbO3 crystals as well as a weak wavefront distortion due to the scattering on dislocation deformation fields. In some images secondary spherical waves were observed as a result of the strong acoustic wave interaction with the submicron size density perturbations.