200 TW peak power has been achieved experimentally using a Cr:forsterite master oscillator at 1250 nm, a stretcher, three optical parametrical amplifiers based on KD*P (DKDP) crystals providing 14.5 J energy in the chirped pulse at 910 nm central wavelength, and a vacuum compressor. The final parametrical amplifier and the compressor are described in detail. Scaling of such architecture to multipetawatt power is discussed.

The pulse spectrum at the laser output was broadened due to self-phase modulation in fused silica and then the pulse was compressed by chirped mirrors. It was demonstrated that with an optimal choice of mirror dispersion a pulse with an energy of 17 J can be compressed from 70 to 14 fs. This compression after compressor approach has undoubted merits: simplicity, low cost, negligible pulse energy losses, and applicability to any high-power laser.

A theoretical model of second-harmonic generation (SHG) under strong influence of cubic nonlinearity was verified in experiment. Effective energy conversion in thin potassium dihydrogen phosphate crystals at peak intensity up to 5 TW/cm² (B-integral equaled 6.4) was demonstrated and no crystal damage was observed. Comparative analysis of SHG of radiation at the fundamental wavelengths of 910 and 800 nm showed the major advantages of the first one. The double-pass geometry of SHG in an ultrathin crystal on a substrate is discussed in detail. Additional correction of parabolic spectral phase of the SH radiation allows pulse duration to be shortened from 20 to 9 fs for 910 nm fundamental wavelength and from 20 to 12 fs for 800 nm.

We discuss the theoretical and experimental investigation of acousto-optic dispersive tunable filters, based on quasi-collinear geometry of light–sound interaction in a tellurium dioxide single crystal. The geometry uses the effect of strong acoustic anisotropy in the paratellurite as well as peculiarities of acoustic wave reflections at the free boundary of the crystal. A mathematical concept for determination of optical, electrical, and constructional parameters of the filters is developed. Different experimental acousto-optic filters intended for femtosecond pulse shaping are designed and tested. Preliminary experiments are performed in a subpetawatt optical parametric chirped pulse amplification laser system. The experimental data conform completely with the predicted data.