We demonstrate intracavity plasmonic laser spectroscopy using a plasmonic laser created from a periodically perforated silver film with a liquid gain medium. An active zone of the laser is formed by a highly elongated spot of pumping. This results in a significantly more efficient diffusive mixing of dye molecules, which suppresses the effect of their bleaching, and in the ability to reduce the volume of the gain medium to as little as 400 nl. We use this design for a stable plasmonic laser in multiple measurements and demonstrate that it is highly effective as a spaser spectroscopy sensor for intracavity detection of an absorptive dye at 0.07 ppm. This work provides an opportunity to develop applications of intracavity plasmonic laser spectroscopy in biological label detection and other fields.
Optical gas sensing attracts growing attention in the recent years. This is governed by progressive availability of optical nanostructures fabrication and complex techniques of optical spectrum processing. In the present paper, a room-temperature optical humidity sensor based on a hydrophilic polymer Nafion is theoretically and experimentally investigated. Sensor geometry is optimized for maximum sensitivity of an angle-resolved ATR dip in the Kretschmann configuration. The reflectance dip is attributed to the 2nd order Nafion layer leaky waveguide mode hybridized with the surface plasmon-polariton at the silver/Nafion interface. Results of the relative humidity (RH) retrieval with the regression of the physical model parameters is compared to these obtained with different machine learning (ML) techniques. It is shown that a limited raw data set is enough for using ML algorithms. Accuracy of 0.3% has been demonstrated in RH measurements.
We show that net amplification of surface plasmons is achieved in channel in a metal plate due to nonradiative excitation by quantum dots. This makes possible lossless plasmon transmission lines in the channel as well as the amplification and generation of coherent surface plasmons. As an example, a ring channel spaser is considered.