The surface and the internal magnetic structure of bamboo-like cylindrical nanowires with tailored diameter modulations have been determined exploiting the direct photoemission and transmission contrasts using photoemission electron microscopy combined with X-ray magnetic circular dichroism, as well as complementary magnetic force microscopy and micromagnetic simulations. Bamboo-like cylindrical nanowires with diameters of 130 and 140 nm, and a modulation periodicity of 400 nm were electrochemically grown into the pores of alumina templates. FeCoCu and Co nanowires were selected to offer parallel and perpendicular magnetization easy axis, respectively. For FeCoCu nanowires, a main longitudinal magnetization configuration is found consistent with the predominant shape anisotropy. In addition, a weaker modulated contrast along the wires’ axis is observed that matches the position of each diameter modulation: vortex-like structures are observed at the ends of the wires and at the surface around the modulations. In Co nanowires, a multi-segmented vortex-like structure with alternating opposite chirality is found not matching the periodicity of the diameter modulations. Such a spin configuration is interpreted considering that Co nanowires exhibit hexagonal symmetry with c axis nearly perpendicular to the nanowires defining strong uniaxial transverse magnetocrystalline anisotropy.

We report a novel pinning type in modulated nanowires: the “corkscrew”. The magnetization in wide segments forms a skyrmion-tube with a helical core along the nanowire.

Cylindrical nanowires synthesized by controlled electrodeposition constitute excellent strategic candidates to engineer magnetic domain configurations. In this work, multisegmented CoNi/Ni nanowires are synthesized for tailoring a periodic magnetic structure determined by the balance between magnetocrystalline and magnetostatic energies. High-resolution Transmission Electron Microscopy confirms the segmented growth and the sharp transition between layers. Although both CoNi and Ni segments have similar fcc cubic crystal symmetry, their magnetic configuration is quite different as experimentally revealed by Magnetic Force Microscopy (MFM) imaging. While the Ni segments are single domain with axial magnetization direction, the CoNi segments present two main configurations: a single vortex state or a complex multivortex magnetic configuration, which is further interpreted with the help of micromagnetic simulations. This original outcome is ascribed to the tight competition between anisotropies. The almost monocrystalline fcc structure of the CoNi segments, as revealed by the electron diffraction patterns, which is atypical for its composition, contributes to balance the magnetocrystalline and shape anisotropies. The results of MFM measurements performed under in-plane magnetic field demonstrate that it is possible to switch from the multivortex configuration to a single vortex configuration with low magnetic fields.

We present experimental evidence of transverse magnetic domains, previously observed only in nanostrips, in CoNi cylindrical nanowires with designed crystal symmetry and tailored magnetic anisotropy. The transverse domains are found together with more conventional vortex domains along the same cylindrical nanowire, denoting a bistable system with similar energies. The surface and the inner magnetization distribution in both types of domains are analyzed by photoemission electron microscopy with x-ray magnetic circular dichroism contrast, and hysteresis loop in individual nanowires are measured by magneto-optical Kerr effect. These experimental data are understood and compared with complementary micromagnetic simulations.

Cylindrical magnetic nanowires show great potential for 3D applications such as magnetic recording, shift registers, and logic gates, as well as in sensing architectures or biomedicine. Their cylindrical geometry leads to interesting properties of the local domain structure, leading to multifunctional responses to magnetic fields and electric currents, mechanical stresses, or thermal gradients. This review article is summarizing the work carried out in our group on the fabrication and magnetic characterization of cylindrical magnetic nanowires with modulated geometry and anisotropy. The nanowires are prepared by electrochemical methods allowing the fabrication of magnetic nanowires with precise control over geometry, morphology, and composition. Different routes to control the magnetization configuration and its dynamics through the geometry and magnetocrystalline anisotropy are presented. The diameter modulations change the typical single domain state present in cubic nanowires, providing the possibility to confine or pin circular domains or domain walls in each segment. The control and stabilization of domains and domain walls in cylindrical wires have been achieved in multisegmented structures by alternating magnetic segments of different magnetic properties (producing alternative anisotropy) or with non-magnetic layers. The results point out the relevance of the geometry and magnetocrystalline anisotropy to promote the occurrence of stable magnetochiral structures and provide further information for the design of cylindrical nanowires for multiple applications.