We have designed and fabricated a custom quartz tuning fork (QTF) with a reduced fundamental frequency; a larger gap between the prongs; and the best quality factor in air at atmospheric conditions ever reported, to our knowledge. Acoustic microresonators have been added to the QTF in order to enhance the sensor sensitivity. We demonstrate a normalized noise equivalent absorption (NNEA) of 3.7 × 10⁻⁹ W.cm⁻¹.Hz^−1/2 for CO₂ detection at atmospheric pressure. The influence of the inner diameter and length of the microresonators has been studied, as well as the penetration depth between the QTF’s prongs. We investigated the acoustic isolation of our system and measured the Allan deviation of the sensor.

We carry out a theoretical investigation of the backward interaction optical parametric oscillator (OPO), in which one of the generated waves is counterpropagating with respect to the pump. We derive simple, self-consistent analytical formulas for the continuous-wave and pulsed regimes. While consistent with previous works on the continuous-wave regime, our study enables us to extend the analysis to the pulsed regime. In particular, we derive simple expressions of the oscillation build-up time, pulsed threshold, and efficiency, for the first time, to our knowledge. We also investigate the peculiar spectral features of the backward OPO when pumped with a narrow-linewidth pulsed radiation, in particular, the absence of tolerance to phase mismatch and the natural ability to emit two waves with a Fourier-transform-limited spectrum. A comparison with the conventional forward OPO is also carried out to emphasize the unique properties of the backward OPO.

We have designed and built a wavelength-tunable optical source for standoff detection of gaseous chemicals by differential absorption spectrometry in the long-wave infrared. It is based on a nanosecond 2 µm single-frequency optical parametric oscillator, whose idler wave is amplified in large aperture Rb:PPKTP crystals. The signal and idler waves are mixed in Z n G e P 2 crystals to produce single-frequency tunable radiation in the 7.5–10.5 µm range. The source was integrated into a direct detection lidar to measure sarin and sulfur mustard inside a closed chamber, in an integrated path configuration with a noncooperative target.

A pulsed, single longitudinal mode, wavelength-tunable Tm:YAP laser is reported. We demonstrate 1 kHz stable operation with 230 µJ, 50 ns pulses and a spectrum linewidth narrowed below 4 pm (FWHM) close to the Fourier transform limit by use of a volume Bragg grating and a YAG etalon. The output wavelength was tuned from 1940 to 1960 nm owing to a transverse chirp of the period of the Bragg grating.

We demonstrate optical parametric amplification in ${\mathrm{ZnGeP}}_2$ (ZGP) of the radiation emitted by a single-frequency continuous-wave quantum cascade laser (QCL) in the range 7.8–8.4 μm. The ZGP amplifier is pumped by a single-frequency parametric source at 2210 nm. For a pump energy of 6 mJ, we report an average gain of 50 over this range and a maximum gain of 111 for 7.5 mJ. An exponential trend is observed when changing the pump energy, with very good agreement with theory. These features are of valuable interest for increasing the standoff detection range of hazardous chemicals and explosives by QCL-based backscattering spectroscopy systems.

We present a differential absorption lidar (DIAL) laser transmitter concept designed around a Nested Cavity Optical Parametric Oscillator (NesCOPO) based Master Oscillator Power Amplifier (MOPA). The spectral bands are located around 2051 nm for CO₂ probing and 1982 nm for H₂¹⁶O and HD¹⁶O water vapor isotopes. This laser is aimed at being integrated into an airborne lidar, intended to demonstrate future spaceborne instrument characteristics: high-energy (several tens of mJ nanosecond pulses) and high optical frequency stability (less than a few hundreds of kHz long term drift). For integration and efficiency purposes, the proposed design is oriented toward the use of state-of-the-art high aperture periodically poled nonlinear materials. This approach is supported by numerical calculations and preliminary experimental validations, showing that it is possible to achieve energies in the 40–50 mJ range, reaching the requirement levels for spaceborne Integrated Path Differential Absorption (IPDA) measurements. We also propose a frequency referencing technique based on beat note measurement of the laser signal with a self-stabilized optical frequency comb, which is expected to enable frequency measurement precisions better than a few 100 kHz over tens of seconds integration time, and will then be used to feed the cavity locking of the NesCOPO.