The use of flawed excavated-mass aggregates produced from crushing and screening hydraulic engineering waste in concrete projects can reduce natural resource extraction, increase waste utilization rates, and minimize environmental pollution. However, the direct application of flawed excavated-mass aggregates is limited due to their high crushing index and water absorption rate. Therefore, this paper measures the multi-dimensional physical and mechanical properties of defective aggregates. A strengthening slurry is prepared by comprehensively modifying the crystallization strength and penetration path of sodium silicate solution using various chemical reagents. The strengthening mechanism of the slurry on flawed excavated-mass aggregates is analyzed using SEM and MIP tests. Concrete tests are designed to investigate the workability and mechanical properties of flawed excavated-mass aggregate concrete. The pore structure of the ITZ (Interfacial Transition Zone) in defective aggregate concrete is analyzed through BSE (Backscattered Electron) imaging to elucidate the strengthening mechanism of secondary crystallization reactions on the ITZ. The research findings can provide technical support for repairing aggregates with defects.