The results of the research and design of a novel vacuum photosensor with a planar molybdenum blade structure are presented. The advanced prototype implements the principle of an increasing penetrability of the Schottky barrier for the metal–vacuum interfaces under the action of an external strong electrostatic field. Theoretical and experimental substantiation of the photosensor performance in a wide range of wavelengths (from 430 to 680 nm and from 800 to 1064 nm) beyond the threshold of the classical photoelectric effect is given. The finite element method was applied to calculate distribution of the optical and electrostatic fields inside the photosensor structure. The sensor current-to-light response was studied using the periodic pulsed irradiation with the tunable wavelength. It was shown that the nanoscale localization zones of two types are formed near the surface of the blade tip: the zone of an increased concentration of hot electrons localized inside the molybdenum blade, and the zone with an increased strength of the external electrostatic field localized outside the blade. In general, the mutual positions of these zones may not coincide, whereas the position of the first-type localization zone significantly varies with the changes in the wavelength of the irradiating light. This causes features in the spectrum of the quantum yield of the photosensor such as expressed non-monotonic behavior and occurrence of sharp dips. The design of the photosensor that provides matching of the positions for both types of localization zones was proposed; the manufactured prototypes of the designed device were experimentally studied. In the designed photosensor, the ballistic transport of photoelectrons in the vacuum gap with a strong field provides a possibility for the creation of ultra-fast optoelectronic devices, such as modulators, detectors, and generators.
The main goal of this work was to modify the previously developed blade-type planar structure using plasmonic gold nanostars in order to stimulate photofield emission and provide efficient laser control of the electron current. Localization and enhancement of the field at the tips of gold nanostars provided a significant increase in the tunneling electron current in the experimental sample (both electrical field and photofield emission). Irradiation at a wavelength in the vicinity of the plasmon resonance (red laser) provided a gain in the photoresponse value of up to 5 times compared to irradiation far from the resonance (green laser). The prospects for transition to regimes of structure irradiation by femtosecond laser pulses at the wavelength of surface plasmon resonance, which lead to an increase in the local optical field, are discussed. The kinetics of the energy density of photoinduced hot and thermalized electrons is estimated. The proposed laser-controlled matrix current source is promising for use in X-ray computed tomography systems.
An important direction in the development of X-ray computed tomography sensors in systems with increased scanning speed and spatial resolution is the creation of an array of miniature current sources. In this paper, we describe a new material based on gold nanostars (GNS) embedded in nanoscale diamond-like carbon (DLC) films (thickness of 20 nm) for constructing a pixel current source with photoinduced electron emission. The effect of localized surface plasmon resonance in GNS on optical properties in the wavelength range from UV to near IR, peculiarities of localization of field and thermal sources, generation of high-energy hot electrons, and mechanisms of their transportation in vacuum are investigated. The advantages of the proposed material and the prospects for using X-ray computed tomography in the matrix source are evaluated.
Anomalous transition to the regime of dynamic chaos in a multimode quantum-well heterolaser (λ = 635 nm) is possible as a result of an injection-current-induced change in the gain. A stable multimode regime (featuring more than ten longitudinal modes) is established near the lasing threshold under conditions of weak nonlinear coupling. As the injection current increases, the competition of modes results in a partial suppression of weak laser modes. At a certain excess of the gain over losses, a regime with hard excitation of four modes is realized that is characterized by the onset of a dynamic chaos manifested by irregular amplitude pulsation of modes, broadening of the optical spectrum, and loss of coherence. The loss of coherence is revealed by a decrease in the visibility of interference bands and by their chaotic shifts. An increase in the overall nonlinear coupling and the corresponding competition of modes leads to a decrease in the dimension of the self-oscillatory system and to the onset of a stable single-mode lasing regime.
Dynamic characteristics of the optovoltaic effect in the mega-and gigahertz range have been studied by detecting longitudinal modes of a semiconductor injection laser diode with a tunable external resonator. The electron lifetime in the active region of the p-n junction was determined by measuring the amplitude of the alternating injection current component at an intermode beat frequency in the course of resonator length tuning. As the resonator length was varied from 1 m to 3 cm, the beat frequency changed from 150 MHz to 5 GHz. In this case, the characteristic range of the optovoltaic effect in GaAlAs laser diodes (λ = 0.82 μm) is limited by the spontaneous electron recombination time, which is on the order of 0.8 ns. An electron-photon noise resonance has been observed in the coherent radiation and in the injection current.
Metal-enhanced fluorescence (MEF) has found widespread application in biomedical sensing and in vivo tissue imaging systems. To enhance MEF efficiency, it is necessary to optimize the interaction between metal nanoparticle plasmon and the fluorophore molecule. The size and shape of the nanoparticle, the nanoscale gap between the fluorescent molecule and the nanoparticle, and the excitation wavelength are critical parameters. In this study, we propose a model for a more complete and accurate description of the processes of molecular excitation and generation of the fluorescence spectral response, introducing new concept of effective properties for field enhancement factor, quantum yield, and fluorescence enhancement factor. The influence of the spectral properties of both the nanostructure plasmon and the fluorophore molecule on the optimal tuning of fluorescent complexes is studied. Particular attention is paid to the analysis of the spectral properties of plasmon resonance and calculations of the near-field intensity enhancement of the plasmonic nanostructure's excitation field. Numerical results for optimizing the MEF of fluorescent complexes based on TagRFP and gold (silver) nanorods composites are presented. The advantages of the proposed model for the optimal design of new nanomaterials with unique fluorescent properties are discussed.