Larry Di Girolamo

Dr. Larry Di Girolamo


Research Focus & Metrics

Academic Career Length

20Years (2007-Present)

(Calculated once Scilit publication data is synced: current year − year of first publication + 1)

Representative Publications

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2 May 2021 in Journal of Geophysical Research: Atmospheres
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AMArka Mitra
Arka Mitra
LGLarry Di Girolamo
Larry Di Girolamo
YHYulan Hong
Yulan Hong
YZYizhe Zhan
Yizhe Zhan
KMKevin J. Mueller
Kevin J. Mueller
Cloud‐top heights (CTH) from the Multiangle Imaging Spectroradiometer (MISR) and the Moderate Resolution Imaging Spectroradiometer (MODIS) on Terra constitute our longest‐running single‐platform CTH record from a stable orbit. Here, we provide the first evaluation of the Terra Level 2 CTH record against collocated International Space Station Cloud‐Aerosol Transport System (CATS) lidar observations between 50ºN and 50ºS. Bias and precision of Terra CTH relative to CATS is shown to be strongly tied to cloud horizontal and vertical heterogeneity and altitude. For single‐layered, unbroken, optically thick clouds observed over all altitudes, the uncertainties in MODIS and MISR CTH are −540 ± 690 m and −280 ± 370 m, respectively. The uncertainties are generally smaller for lower altitude clouds and larger for optically thin clouds. For multi‐layered clouds, errors are summarized herein using both absolute CTH and CATS‐layer‐altitude proximity to Terra CTH. We show that MISR detects the lower cloud in a two‐layered system, provided top‐layer optical depth <∼0.3, but MISR low‐cloud CTH errors are unaltered by the presence of thin cirrus. Systematic and random errors are propagated to explain inter‐sensor disagreements, as well as to provide the first estimate of the MISR stereo‐opacity bias. For MISR, altitude‐dependent wind‐retrieval bias (−90 to −110 m) and stereo‐opacity bias (−60 to −260 m) and for MODIS, CO2‐slicing bias due to geometrically thick cirrus leads to overall negative CTH bias. MISR’s precision is largely driven by precision in retrieved wind‐speed (3.7 m s−1), whereas MODIS precision is driven by forward‐modeling uncertainty.

12 December 2019 in Journal of Geophysical Research: Atmospheres
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MFMichael Fromm
Michael Fromm
DPDavid Peterson
David Peterson
LGLarry Di Girolamo
Larry Di Girolamo
The literature‐‐spanning several recent decades‐‐describes numerous attempts to characterize the efficacy of cumulonimbus “Cb” convection as a pollutant pathway connecting the planetary BL to the upper troposphere and lower stratosphere (UTLS). The relatively new discovery of wildfires triggering deep convection and Cb formation, referred to as pyrocumulonimbus “pyroCb”, has provided a new convective candidate for examination. Previous studies have shown that the pyroCb pathway offers a reinterpretation of supposed volcanic aerosol layers observed in the stratosphere. The community now questions whether this relatively unappreciated phenomenon has been overlooked or imprecisely characterized in published analyses of observed UTLS biomass burning constituents attributed to traditional convection, such as individual Cbs or larger mesoscale convective systems. Here we show that on at least two occasions, a reinterpretation of the literature is required. Both are in the context of coordinated measurement campaigns in summertime Central and North American domains. We provide a strategic review of prior studies and explore three selected works, wherein the pyroCb naturally explains observations of dramatically strong, remote, and high‐altitude biomass burning pollution. We complete our discussion with the implications for including the pyroCb phenomenon in case studies and assessments of the primary convective pathway for smoke particles to enter the UTLS.

27 June 2022 in Atmospheric Chemistry and Physics
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DFDongwei Fu
Dongwei Fu
LGLarry Di Girolamo
Larry Di Girolamo
RRRobert M. Rauber
Robert M. Rauber
GMGreg M. McFarquhar
Greg M. McFarquhar
SNStephen W. Nesbitt
Stephen W. Nesbitt
ASAmy Jo Scarino
Amy Jo Scarino
The cloud drop effective radius (Re) of the drop size distribution derived from passive satellite sensors is a key variable used in climate research. Validation of these satellite products has often taken place under stratiform cloud conditions that favor the assumption of cloud horizontal homogeneity used by the retrieval techniques. However, many studies have noted concerns with respect to significant biases in retrieved Re arising from cloud heterogeneity, for example, in cumulus cloud fields. Here, we examine data collected during the 2019 “Cloud, Aerosol and Monsoon Processes Philippines Experiment” (CAMP2Ex), which, in part, targeted the objective of providing the first detailed evaluation of Re retrieved across multiple platforms and techniques in a cumulus and congestus cloud region. Our evaluation consists of cross-comparisons of Re between the Moderate Resolution Imaging Spectroradiometer (MODIS) onboard the Terra satellite, the Research Scanning Polarimeter (RSP) onboard the NASA P-3 aircraft, and in situ measurements from both the NASA P-3 and Learjet aircraft that are all taken in close spatiotemporal proximity to the same cloud fields. A particular advantage of our approach lies in the capability of the RSP to retrieve Re using a bi-spectral MODIS approach and a polarimetric approach, which allows for the evaluation of bi-spectral and polarimetric Re retrievals from an airborne perspective using the same samples. Averaged over all P-3 flight segments examined here for warm clouds, the RSP polarimetric method, the in situ method, and the bias-adjusted MODIS method of Fu et al. (2019) show a comparable median (mean ± standard deviation) for the Re samples of 9.6 (10.2 ± 4.0) µm, 11.0 (13.6 ± 11.3) µm, and 10.4 (10.8 ± 3.8) µm, respectively. These values are far lower than the values of 15.1 (16.2 ± 5.5) µm and 17.2 (17.7 ± 5.7) µm from the bi-spectral retrievals of RSP and MODIS, respectively. Similar results are observed when Re is segregated by cloud-top height and in detailed case studies. The clouds sampled during CAMP2Ex consist of mostly small (mean transect length ∼ 1.4 km) and low clouds (mean cloud-top height ∼ 1 km), which had more numerous small clouds than the trade wind cumuli sampled in past field campaigns such as Rain in Shallow Cumulus over the Ocean (RICO) and the Indian Ocean Experiment (INDOEX). The overestimates of Re from the RSP bi-spectral technique compared with the polarimetric technique increased as cloud size and cloud optical depth decreased. Drizzle, cloud-top bumpiness, and solar zenith angle, however, are not closely correlated with the overestimate of bi-spectral Re. For shallow clouds that dominated the liquid cloud cover for the CAMP2Ex region and period, we show that 3-D radiative transfer and cloud heterogeneity, particularly for the optically thin and small clouds, appear to be the leading cause of the large positive biases in bi-spectral retrievals. Because this bias varies with the underlying structure of the cloud field, caution continues to be warranted in studies that use bi-spectral Re retrievals in cumulus cloud fields.

8 December 2019 in Journal of Geophysical Research: Atmospheres
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DFDongwei Fu
Dongwei Fu
LGLarry Di Girolamo
Larry Di Girolamo
LLLusheng Liang
Lusheng Liang
GZGuangyu Zhao
Guangyu Zhao
Satellite measurements from Terra's Moderate Resolution Imaging Spectroradiometer (MODIS) represent our longest, single‐platform, global record of the effective radius (Re) of the cloud drop size distribution. Quantifying its error characteristics has been challenging because systematic errors in retrieved Re covary with the structural characteristics of the cloud and the Sun‐view geometry. Recently, it has been shown that the bias in MODIS Re can be estimated by fusing MODIS data with data from Terra's Multi‐angle Imaging SpectroRadiometer (MISR). Here, we relate the bias to the observed underlying conditions to derive regional‐scale, bias‐corrected, monthly‐mean Re1.6, Re2.1, and Re3.7 values retrieved from the 1.6, 2.1, and 3.7 μm MODIS spectral channels. Our results reveal that monthly‐mean bias in Re2.1 exhibits large regional dependency, ranging from at least ~1 to 10 μm (15 to 60%) varying with scene heterogeneity, optical depth, and solar zenith angle. Regional bias‐corrected monthly‐mean Re2.1 ranges from 4 to 17 μm, compared to 10 to 25 μm for uncorrected Re2.1, with estimated uncertainties of 0.1 to 1.8 μm. The bias‐corrected monthly‐mean Re3.7 and Re2.1 show difference of approximately +0.6 μm in the coastal marine stratocumulus regions and down to approximately −2 μm in the cumuliform cloud regions, compared to uncorrected values of about −1 to −6 μm, respectively. Bias‐corrected Re values compare favorably to other independent data sources, including field observations, global model simulations, and satellite retrievals that do not use retrieval techniques similar to MODIS. This work changes the interpretation of global Re distributions from MODIS Re products and may further impact studies, which use the original MODIS Re products to study, for example, aerosol‐cloud interactions and cloud microphysical parameterization.

16 July 2020 in Atmospheric Chemistry and Physics
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YHYulan Hong
Yulan Hong
LGLarry Di Girolamo
Larry Di Girolamo
This study examines the climatology of cloud phase over Southeast Asia (SEA) based on A-Train satellite observations. Using the combined CloudSat–CALIPSO (CC) data, five main cloud groups are investigated: ice-only, ice-above-liquid, liquid-only, ice-above-mixed, and mixed-only clouds that have annual mean frequencies of 28.6 %, 20.1 %, 16.0 %, 9.3 %, and 6.7 %, respectively. Liquid-only clouds tend to occur in relatively cold, dry, and stable lower troposphere. The other four cloud groups appear more frequently in relatively warm, humid, and unstable conditions, and their seasonal distributions move with the Asian monsoon and the Intertropical Convergence Zone (ITCZ). Liquid clouds are found to be highly inhomogeneous based on the heterogeneity index (Hσ) from Aqua Moderate Resolution Imaging Spectroradiometer (MODIS), while ice-only and mixed-only clouds are often very smooth. Ice-above-liquid clouds are more heterogeneous than ice-only clouds owing to ice clouds being optically thin. We demonstrate that the distribution of clear-sky Hσ has a long tail towards heterogeneous values that are caused by undetected subpixel cloud within both CC and MODIS datasets. The reflectance at 0.645 µm (R0.645) and brightness temperature at 11 µm (BT11) of CC ice-only, liquid-only, and ice-above-liquid clouds show peak frequencies near that of clear sky (R0.645∼0.02; BT11∼294 K), which explains why up to 30 % of these CC cloud groups are classified as clear by MODIS. In contrast, mixed-only clouds are thick (average top ∼13 km), bright (average R0.645∼0.6), and cold (average BT11 ∼234 K). Cloud phase comparison between CC and MODIS reveals only modest agreement, with the best agreement (73 %) occurring between CC ice-above-mixed and MODIS ice clouds. The intraseasonal and interannual behaviors of the all-sky Hσ and spectral signatures follow that of cloud phase and vary with the Madden–Julian oscillation (MJO) and the El Niño–Southern Oscillation (ENSO) phases.

11 August 2023 in Atmospheric Chemistry and Physics
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RMRose Marie Miller
Rose Marie Miller
RRRobert M. Rauber
Robert M. Rauber
LGLarry Di Girolamo
Larry Di Girolamo
MRMatthew Rilloraza
Matthew Rilloraza
DFDongwei Fu
Dongwei Fu
KTKenneth Lee Thornhill
Kenneth Lee Thornhill
Cumulus clouds are common over maritime regions. They are important regulators of the global radiative energy budget and global hydrologic cycle, as well as a key contributor to the uncertainty in anthropogenic climate change projections due to uncertainty in aerosol–cloud interactions. These interactions are regionally specific owing to their strong influences on aerosol sources and meteorology. Here, our analysis focuses on the statistical properties of marine boundary layer (MBL) aerosol chemistry and the relationships of MBL aerosol to cumulus cloud properties just above cloud base as sampled in 2019 during the NASA Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex). The aerosol and clouds were sampled by instruments on the NASA P-3 aircraft over three distinct maritime regions around the Philippines: the West Pacific, the South China Sea, and the Sulu Sea. Our analysis shows three primary sources influenced the aerosol chemical composition: clean marine (ocean source), industrial (Southeast Asia, Manila, and cargo and tanker ship emissions), and biomass burning (Borneo and Indonesia). The clean marine aerosol chemical composition had low values of all sampled chemical signatures, specifically median values of 2.2 µg m−3 of organics (ORG), 2.3 µg m−3 of SO4, 0.3 µg m−3 of NO3, 1.4 µg m−3 of NH4, 0.04 µg m−3 of Cl, and 0.0074 µg m−3 of refractory black carbon (BC). Chemical signatures of the other two aerosol source regions were industrial, with elevated SO4 having a median value of 6.1 µg m−3, and biomass burning, with elevated median concentrations of ORG 21.2 µg m−3 and BC 0.1351 µg m−3. Based on chemical signatures, the industrial component was primarily from ship emissions, which were sampled within 60 km of ships and within projected ship plumes. Normalized cloud droplet size distributions in clouds sampled near the MBL passes of the P-3 showed that clouds impacted by industrial and biomass burning contained higher concentrations of cloud droplets, by as much as 1.5 orders of magnitude for diameters < 13 µm compared to clean marine clouds, while at size ranges between 13.0–34.5 µm the median concentrations of cloud droplets in all aerosol categories were nearly an order of magnitude less than the clean marine category. In the droplet size bins centered at diameters > 34.5 µm concentrations were equal to, or slightly exceeded, the concentrations of the clean marine clouds. These analyses show that anthropogenic aerosols generated from industrial and biomass burning sources significantly influenced cloud base microphysical structure in the Philippine region enhancing the small droplet concentration and reducing the concentration of mid-sized droplets.