Yannick Lorgouilloux

Dr. Yannick Lorgouilloux


Research Focus & Metrics

Academic Career Length

21Years (2006-Present)

(Calculated once Scilit publication data is synced: current year − year of first publication + 1)

Representative Publications

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30 September 2021 in Materials Advances
Verified
Journal Article
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BYBakytzhan Yeskendir
Bakytzhan Yeskendir
JDJean-Philippe Dacquin
Jean-Philippe Dacquin
YLYannick Lorgouilloux
Yannick Lorgouilloux
CCChristian Courtois
Christian Courtois
Sebastien RoyerSebastien Royer
Sebastien Royer
JDJérémy Dhainaut
Jérémy Dhainaut
Metal–organic frameworks represent a class of porous materials which have developed considerably over the past few years. Their highly porous structure makes them outperform conventional adsorbents in hot topics such as dihydrogen and methane storage, and carbon dioxide capture. Their consequent modularity, based on the assembly of organic linkers and metal ions or clusters, also brings novel perspectives in catalysis, sensing and drug delivery just to name a few. However, one of the main bottlenecks to their broader use remains their shaping. Especially, shaped materials should present long-term mechanical stability as well as preserve their physical and chemical properties. This makes shaping of MOFs a special case as their thermal and chemical stabilities remain a downside as compared to other traditional porous materials such as silicas and zeolites today. Therefore, ever-increasing efforts have been devoted to the shaping of these materials. In this review, the state of the art for the preparation of shaped 3D MOF-based materials will be presented. Emphasis will be given to the final physical and chemical properties of the shaped solids comparatively to the initial powders, when data are available. In the first part, traditional techniques based on applying a significant force to MOF-based powders will be reviewed. These include pelletization, granulation, and extrusion, which generally lead to an increase of the final volumetric gas uptake of the objects. At the same time, the advantages and disadvantages of each technique will be discussed as well as the main outcome on the final objects. In the second part, the focus will be on newly-emerging techniques such as 3D printing and spray drying. The former also maximizes the volumetric gas uptake of the final materials, and for both techniques the quality of the final objects heavily relies on the working parameters. Finally, the third part will include the so-called “phase separation” shaping techniques which are for the most part performed without using special techniques. This implies shaping via physical and chemical phenomena such as sublimation and precipitation. Subsequently, a discussion on the performance of these materials for adsorption-based applications will be provided. Finally, perspectives and future outlook will be discussed.

1 July 2009 in Journal of Catalysis
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Journal Article
Closed access
BGB.C. Gagea
B.C. Gagea
YLYannick Lorgouilloux
Yannick Lorgouilloux
YAY. Altintas
Y. Altintas
PJP.A. Jacobs
P.A. Jacobs
JMJohan Martens
Johan Martens

12 April 2013 in Langmuir
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Journal Article
Closed access
TRTom Remy
Tom Remy
SPSunil A. Peter
Sunil A. Peter
LTLeen Van Tendeloo
Leen Van Tendeloo
SPStijn Van der Perre
Stijn Van der Perre
YLYannick Lorgouilloux
Yannick Lorgouilloux
JDJoeri F. M. Denayer
Joeri F. M. Denayer

13 July 2010 in Journal of the American Chemical Society
Verified
Journal Article
Closed access
MDMathias Dodin
Mathias Dodin
JPJean-Louis Paillaud
Jean-Louis Paillaud
YLYannick Lorgouilloux
Yannick Lorgouilloux
PCPhilippe Caullet
Philippe Caullet
EEErik Elkaïm
Erik Elkaïm
NBNicolas Bats
Nicolas Bats

1 March 2009 in Journal of Solid State Chemistry
Verified
Journal Article
Closed access
YLYannick Lorgouilloux
Yannick Lorgouilloux
MDMathias Dodin
Mathias Dodin
JPJean-Louis Paillaud
Jean-Louis Paillaud
PCPhilippe Caullet
Philippe Caullet
LMLaure Michelin
Laure Michelin
NBNicolas Bats
Nicolas Bats

28 October 2006 in Journal of Materials Science
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Journal Article
Closed access
PDF file
EFE. Yeugo Fogaing
E. Yeugo Fogaing
YLYannick Lorgouilloux
Yannick Lorgouilloux
MHM. Huger
M. Huger
CGC. P. Gault
C. P. Gault