Organic–inorganic hybrid perovskites (OIHPs) have been widely used in fields such as solar cells, photodetectors, and light-emitting diodes due to their simple preparation by solution methods and excellent optoelectronic properties. In recent years, numerous scholars have delved deeply into the magneto-optical properties of perovskites and explored their potential applications in the magneto-optical field. Herein, we present the Faraday rotation characteristics of formamidinium lead bromide (Fabri₃) single crystals within the visible spectrum range. Firstly, FAPbBr₃ single crystals with high transparency and a size of 5.5 × 5.6 × 2 mm³ were prepared using the modified inverse temperature crystallization (MITC) method. The experimental results showed that the Verdet constant of FAPbBr₃ single crystal at 565 nm was up to 531.6 rad/(T·m). Furthermore, the FAPbBr₃ single crystal showed similar or an even higher Verdet constant when compared with the mature magneto-optical material TGG single crystal commonly used in the industry. The thermal simulation results of the FAPbBr₃ single crystal show low temperature dependence which achieves about 90% isolation transparency with a magnetic field of 0.35 T for 625 nm. This study demonstrates the outstanding Faraday rotation properties of FAPbBr₃ single crystals, thereby offering promising prospects for the development of perovskite materials in non-reciprocal devices such as optical isolators and optical circulators.