Altermagnetism represents an emergent collinear magnetic phase with compensated order and an unconventional alternating even-parity wave spin order in the non-relativistic band structure. We investigate directly this unconventional band splitting near the Fermi energy through spin-integrated soft X-ray angular resolved photoemission spectroscopy. The experimentally obtained angle-dependent photoemission intensity, acquired from epitaxial thin films of the predicted altermagnet CrSb, demonstrates robust agreement with the corresponding band structure calculations. In particular, we observe the distinctive splitting of an electronic band on a low-symmetry path in the Brilliouin zone that connects two points featuring symmetry-induced degeneracy. The measured large magnitude of the spin splitting of approximately 0.6 eV and the position of the band just below the Fermi energy underscores the significance of altermagnets for spintronics based on robust broken time reversal symmetry responses arising from exchange energy scales, akin to ferromagnets, while remaining insensitive to external magnetic fields and possessing THz dynamics, akin to antiferromagnets.
The anomalous Nernst effect generates a voltage transverse to an applied thermal gradient in some magnetically ordered systems. While the effect was considered excluded in compensated magnetic materials with collinear ordering, in the recently identified symmetry-class of altermagnets, the anomalous Nernst effect is possible despite the compensated collinear spin arrangement. In this work, we show that epitaxial Mn5Si3 thin films grown on Si manifest an anomalous Nernst effect with a finite spontaneous signal at zero magnetic field despite the vanishing spontaneous magnetization. We attribute this to the previously theoretically predicted and experimentally corroborated altermagnetism of epitaxial Mn5Si3 thin films grown on Si. The observed spontaneous anomalous Nernst coefficient reaches the value of 0.26 μV/K with the corresponding spontaneous Nernst conductivity of 0.22 A/(K ⋅ m). To complement our measurements, we perform density-functional theory calculations of the momentum-resolved anomalous Nernst conductivity, highlighting the contributions of altermagnetic pseudonodal surfaces and ladder transitions to the Berry curvature. Our results illustrate the value of unconventional d-wave wave altermagnets composed of abundant and non-toxic light elements for thermo-electrics and spin-caloritronics.
Investigating the off-diagonal components of the conductivity and thermoelectric tensor of materials hosting complex antiferromagnetic structures has become a viable method to reveal the effects of topology and chirality on the electronic transport in these systems. In this respect, Mn5Si3 is an interesting metallic compound that exhibits several antiferromagnetic phases below 100 K with different collinear and noncollinear arrangements of Mn magnetic moments determined from neutron scattering. Previous electronic transport measurements have shown that the transitions between the various phases give rise to large changes of the anomalous Hall effect. Here, we report measurements of the anomalous Nernst effect of Mn5Si3 single crystals that also show clear transitions between the different magnetic phases. In the noncollinear phase, we observe an unusual sign change of the zero-field Nernst signal with a concomitant decrease of the Hall signal and a gradual reduction of the remanent magnetization. Furthermore, a symmetry analysis of the proposed magnetic structures shows that both effects should actually vanish. These results indicate a symmetry-breaking modification of the magnetic state with a rearrangement of the magnetic moments at low temperatures, thus questioning the previously reported models for the noncollinear magnetic structure obtained from neutron scattering.
Reflection and refraction of light can be used to trap small dielectric particles in the geometrical optics regime. Absorption of light is usually neglected in theoretical calculations, but it is known that it occurs in the optical trapping of semi-transparent particles. Here, we propose a generalization of Ashkin’s model for the radiative force exerted on a spherical bead, including the contribution due to attenuation/absorption of light in the bulk of the particle. We discuss in detail the balance between refraction, reflection, and absorption for different optical parameters and particle sizes. Our findings contribute to the understanding of optical trapping of light-absorbing particles and may be used to predict whenever absorption is important in real experiments.
Altermagnetism, a recently proposed and experimentally confirmed class of magnetic order, features collinear compensated magnetism with unconventional spin-split bands. Here, we show that in a metallic 2D d -wave altermagnet with [ C 2 | | C 4 ] symmetry, secondary instabilities can arise. Using an unbiased functional renormalization group approach, we analyze the weak-coupling instabilities of a 2D Hubbard model with a preexisting altermagnetic order inspired by our electronic structure calculations of realistic material candidates from V 2 X 2 O ( X = Te, Se) family. We identify two distinct spin-density-wave (SDW) states that break the underlying altermagnetic [ C 2 | | C 4 ] symmetry. Additionally, we find spin-fluctuation-induced instabilities leading to a singlet d -wave superconducting state and an unconventional commensurate pair-density-wave (PDW) state with extended s -wave and spin-triplet symmetry. We analyze the pairing mechanism and characterize the excitation spectrum, which exhibits Bogoliubov Fermi surfaces or nodal points depending on the gap size.