A comprehensive experimental investigation of exciton and biexciton recombination in GaAs/AlGaAs quantum wells is presented. Exciton and biexciton recombination times are found to be 16 and 55 ps, respectively. A method of determining the dynamics of the exciton temperature is developed. It is shown that both exciton and biexciton recombination processes increase the exciton temperature by an amount as high as K. These processes impose a new restriction on the possibility of exciton Bose-Einstein condensation and make impossible its achievement in a system of direct excitons in GaAs quantum wells even for resonantly excited exciton gas.
We study photoluminescence (PL) spectra and exciton dynamics of the MoS2 monolayer (ML) grown by the chemical vapor deposition technique. In addition to the usual direct A-exciton line, we observe a low-energy line of bound excitons dominating the PL spectra at low temperatures. This line shows unusually strong redshift with an increase in the temperature and submicrosecond time dynamics suggesting indirect nature of the corresponding transition. By monitoring the temporal dynamics of exciton PL distribution in the ML plane, we observe diffusive transport of A-excitons and measure the diffusion coefficient up to 40 cm2/s at elevated excitation powers. The bound exciton spatial distribution spreads over tens of micrometers in μs. However, this spread is subdiffusive, characterized by a significant slowing down with time. The experimental findings are interpreted as a result of the interplay between the diffusion and Auger recombination of excitons.
The dynamics of excitons and trions in GaAs/AlGaAs heterostructures with shallow quantum wells is studied in time-resolved photoluminescence experiments carried out with different repetition rates of picosecond pump pulses for the cases of intrawell, above-barrier, and“two-color” excitation. It is established that excess charge carriers of one type accumulated in the quantum wells under above-barrier excitation play a key role in the formation and dynamics of the exciton-trion system and determine its composition and kinetic properties. The lifetime of excess charge carriers in the quantum wells, estimated from the experimental data, exceeds 10 μs.
We study the spin dynamics in a high-mobility two-dimensional electron gas confined in a GaAs/AlGaAs quantum well. An unusual magnetic field dependence of the spin relaxation is found: As the magnetic field becomes stronger, the spin relaxation time first increases quadratically but then changes to a linear dependence before it eventually becomes oscillatory, whereby the longitudinal and transverse times reach maximal values at even and odd filling Landau level factors, respectively. We show that the suppression of spin relaxation is due to the effect of electron gyration on the spin-orbit field, while the oscillations correspond to oscillations of the density of states appearing at low temperatures and high magnetic fields. The transition from quadratic to linear dependence can be related to a transition from classical to Bohm diffusion and reflects an anomalous behavior of the two-dimensional electron gas analogous to that observed in magnetized plasmas.