The structure and nature of the crust underlying the Santos Basin‐São Paulo Plateau System (SSPS), in the SE Brazilian margin, are discussed based on five wide‐angle seismic profiles acquired during the Santos Basin (SanBa) experiment in 2011. Velocity models allow us to precisely divide the SSPS in six domains from unthinned continental crust (Domain CC) to normal oceanic crust (Domain OC). A seventh domain (Domain D), a triangular shape region in the SE of the SSPS, is discussed by Klingelhoefer et al. (2014). Beneath the continental shelf, a ~100 km wide necking zone (Domain N) is imaged where the continental crust thins abruptly from ~40 km to less than 15 km. Toward the ocean, most of the SSPS (Domains A and C) shows velocity ranges, velocity gradients, and a Moho interface characteristic of the thinned continental crust. The central domain (Domain B) has, however, a very heterogeneous structure. While its southwestern part still exhibits extremely thinned (7 km) continental crust, its northeastern part depicts a 2–4 km thick upper layer (6.0–6.5 km/s) overlying an anomalous velocity layer (7.0–7.8 km/s) and no evidence of a Moho interface. This structure is interpreted as atypical oceanic crust, exhumed lower crust, or upper continental crust intruded by mafic material, overlying either altered mantle in the first two cases or intruded lower continental crust in the last case. The deep structure and v‐shaped segmentation of the SSPS confirm that an initial episode of rifting occurred there obliquely to the general opening direction of the South Atlantic Central Segment.

During the Sanba (Santos basin seismic transect) experiment in 2010–2011, a 380-km-long combined wide-angle and reflection seismic profile has been acquired using 30 ocean-bottom seismometers, a 4.5 km seismic streamer and a 8900 in.³ airgun array. The Sanba 3 profile crosses the southern flank of the Sao Paulo Plateau, the Sao Paulo Ridge and the easternmost Santos Basin in an east–west direction. Its eastern end is located on undisturbed oceanic crust. Tomographic and forward modelling of the wide-angle seismic data reveals that the sedimentary thickness is variable with only 1–2 km on top of the ridge and thickening to 4–5 km in the basin. Crustal thickness at the ridge is about 18 km and the relative layer thickness and velocity gradients indicate a continental origin of this ridge. The eastern Santos Basin is underlain by crust of only 5 km thickness, characterized by high seismic velocities between 6.20 km s^–1 in the upper crust and 7.40 km s^–1 in the lower crust. Three hypotheses for the nature of the crust in this region are tested here: (i) thinned continental crust, (ii) serpentinized upper mantle material, (iii) thin oceanic crust. As seismic velocity gradients seem to rule out a continental origin of this region, and clear Moho reflections argue against serpentinized upper mantle, we propose that the crust underlying the easternmost Santos Basin is of oceanic origin. Deviations from normal oceanic crustal velocities in the lower crust (6.70–7.00 km s^–1) can be explained by accretion at slow spreading rates leading to the inclusion of serpentinite into the lower crust at the onset of organized seafloor spreading.

The North Natal Valley (NNV) and the Mozambique Coastal Plain (MCP) are key areas for the understanding of the SW Indian Ocean history since the Gondwana break‐up. Nevertheless, the deep structures and the nature of the NNV and MCP remain discussed in the absence of deep geophysical data. In 2016, the NNV, MCP and Limpopo margin (LM) have been investigated along seven wide‐angle and MCS profiles. The combined wide‐angle and reflection seismic interpretation along the N‐S MZ7 profile reveals an upper sedimentary sequence characterized by low velocities generally not exceeding 3 km/s, with thicknesses varying from 0.150 km in the central part to ∼2.8 km in the south. The underlying sequence is formed of a 2.53.0 km thick volcano‐sedimentary sequence which presents important lateral and with depth changes and presence of high velocity lenses, indicating inter‐bedded volcanic sills and recurrent magmatic episodes. The south of the NNV including the Naude Ridge (NR) presents a disturbed sedimentary cover with structural highs and southward‐dipping reflectors and sub‐basins. The crust, reaching 35–40 km onshore below the MCP, gently thins below the continental shelf to a regular thickness of ∼29 km below the NNV. Crustal velocities reveal low velocity gradients, with atypical high velocities. South the ND, the crust thins to 15 km. We interpret the velocity architecture combined with the evidences of volcanism at shallower depths as indicating an intensively intruded continental crust. Contrary to what is proposed in most geodynamic models, the Mozambique Coastal plain and the Natal Valley are both of continental nature, with an abrupt necking zone located south of NR. The Antarctica plate was therefore situated at the eastern limit of these two domains before the Gondwana breakup.