The international journal of Aerosol and Air Quality Research (AAQR) covers all aspects of aerosol science and technology, atmospheric science and air quality related issues.
Recovery and treatment of methane from coal mine ventilation air methane (VAM) with cost-effective technologies have been an ongoing challenge due to low methane concentrations. In this study, a type of coconut shell-based active carbon was employed to enrich VAM with a three-bed vacuum pressure swing adsorption unit. A new vacuum exhaust step for the VPSA process was introduced. The results show that the vacuum exhaust step can increase the methane concentration of the product without changing adsorption and desorption pressure. Under laboratory conditions, the concentration of product increased from 0.4% to 0.69% as the vacuum exhaust ratio increased from 0 to 3.1 when the feed gas concentration was 0.2%. A 500 m³/h pilot-scale test system for VAM enrichment was built rendering good correlation with the laboratory results in terms of the vacuum exhaust step. By using a two-stage three-bed separation unit, the VAM was enriched from 0.2% to over 1.2%.
Radial flow is an important type of flow direction for large-scale pressure swing adsorption (PSA) oxygen generation systems. In this study, a numerical simulation of a PSA oxygen generation process based on radial-flow adsorbers was performed with two-dimensional CFD modeling. The gas distribution, the maldistribution factor and the pressure difference were comparatively investigated at each flow type of the radial-flow adsorber. Considering the gas adsorption performance, the results indicated that the centripetal π-flow radial adsorber has the best flow characteristics for the PSA process. The oxygen purity distribution within the adsorption bed was studied to compare centripetal and centrifugal π-flows, and the former was shown to perform better on oxygen enrichment and adsorbent desorption. The steady state was achieved after eight cycles for the centripetal-π adsorber and each of the four steps of the PSA process was explored in detail to show the advantageous properties for oxygen generation in terms of adsorption and desorption. The relationships between the product flow rate and the oxygen purity and recovery were further investigated.