Variations in solar radiation incident at Earth's surface profoundly affect the human and terrestrial environment. A decline in solar radiation at land surfaces has become apparent in many observational records up to 1990, a phenomenon known as global dimming. Newly available surface observations from 1990 to the present, primarily from the Northern Hemisphere, show that the dimming did not persist into the 1990s. Instead, a widespread brightening has been observed since the late 1980s. This reversal is reconcilable with changes in cloudiness and atmospheric transmission and may substantially affect surface climate, the hydrological cycle, glaciers, and ecosystems.

The literature on atmospheric particulate matter (PM), or atmospheric aerosol, has increased enormously over the last 2 decades and amounts now to some 1500–2000 papers per year in the refereed literature. This is in part due to the enormous advances in measurement technologies, which have allowed for an increasingly accurate understanding of the chemical composition and of the physical properties of atmospheric particles and of their processes in the atmosphere. The growing scientific interest in atmospheric aerosol particles is due to their high importance for environmental policy. In fact, particulate matter constitutes one of the most challenging problems both for air quality and for climate change policies. In this context, this paper reviews the most recent results within the atmospheric aerosol sciences and the policy needs, which have driven much of the increase in monitoring and mechanistic research over the last 2 decades. The synthesis reveals many new processes and developments in the science underpinning climate–aerosol interactions and effects of PM on human health and the environment. However, while airborne particulate matter is responsible for globally important influences on premature human mortality, we still do not know the relative importance of the different chemical components of PM for these effects. Likewise, the magnitude of the overall effects of PM on climate remains highly uncertain. Despite the uncertainty there are many things that could be done to mitigate local and global problems of atmospheric PM. Recent analyses have shown that reducing black carbon (BC) emissions, using known control measures, would reduce global warming and delay the time when anthropogenic effects on global temperature would exceed 2 °C. Likewise, cost-effective control measures on ammonia, an important agricultural precursor gas for secondary inorganic aerosols (SIA), would reduce regional eutrophication and PM concentrations in large areas of Europe, China and the USA. Thus, there is much that could be done to reduce the effects of atmospheric PM on the climate and the health of the environment and the human population. A prioritized list of actions to mitigate the full range of effects of PM is currently undeliverable due to shortcomings in the knowledge of aerosol science; among the shortcomings, the roles of PM in global climate and the relative roles of different PM precursor sources and their response to climate and land use change over the remaining decades of this century are prominent. In any case, the evidence from this paper strongly advocates for an integrated approach to air quality and climate policies.

The energy budgets over land and oceans are still afflicted with considerable uncertainties, despite their key importance for terrestrial and maritime climates. We evaluate these budgets as represented in 43 CMIP5 climate models with direct observations from both surface and space and identify substantial biases, particularly in the surface fluxes of downward solar and thermal radiation. These flux biases in the various models are then linearly related to their respective land and ocean means to infer best estimates for present day downward solar and thermal radiation over land and oceans. Over land, where most direct observations are available to constrain the surface fluxes, we obtain 184 and 306 Wm⁻² for solar and thermal downward radiation, respectively. Over oceans, with weaker observational constraints, corresponding estimates are around 185 and 356 Wm⁻². Considering additionally surface albedo and emissivity, we infer a surface absorbed solar and net thermal radiation of 136 and −66 Wm⁻² over land, and 170 and −53 Wm⁻² over oceans, respectively. The surface net radiation is thus estimated at 70 Wm⁻² over land and 117 Wm⁻² over oceans, which may impose additional constraints on the poorly known sensible/latent heat flux magnitudes, estimated here near 32/38 Wm⁻² over land, and 16/100 Wm⁻² over oceans. Estimated uncertainties are on the order of 10 and 5 Wm⁻² for most surface and TOA fluxes, respectively. By combining these surface budgets with satellite-determined TOA budgets we quantify the atmospheric energy budgets as residuals (including ocean to land transports), and revisit the global mean energy balance.