Recently two emerging areas of research, attosecond and nanoscale physics, have started to come together. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time scales, interact with atoms, molecules or solids. The laser-induced electron dynamics occurs natively on a timescale down to a few hundred or even tens of attoseconds (1 attosecond = 1 as = 10 −18 s), which is comparable with the optical field. For comparison, the revolution of an electron on a 1s orbital of a hydrogen atom is ∼152 as. On the other hand, the second branch involves the manipulation and engineering of mesoscopic systems, such as solids, metals and dielectrics, with nanometric precision. Although nano-engineering is a vast and well-established research field on its own, the merger with intense laser physics is relatively recent. In this report on progress we present a comprehensive experimental and theoretical overview of physics that takes place when short and intense laser pulses interact with nanosystems, such as metallic and dielectric nanostructures. In particular we elucidate how the spatially inhomogeneous laser induced fields at a nanometer scale modify the laser-driven electron dynamics. Consequently, this has important impact on pivotal processes such as above-threshold ionization and high-order harmonic generation. The deep understanding of the coupled dynamics between these spatially inhomogeneous fields and matter configures a promising way to new avenues of research and applications. Thanks to the maturity that attosecond physics has reached, together with the tremendous advance in material engineering and manipulation techniques, the age of atto-nanophysics has begun, but it is in the initial stage. We present thus some of the open questions, challenges and prospects for experimental confirmation of theoretical predictions, as well as experiments aimed at characterizing the induced fields and the unique electron dynamics initiated by them with high temporal and spatial resolution.
We present energy-resolved measurements of electron emission from sharp metal tips driven with low energy pulses from a few-cycle laser oscillator. We observe above-threshold photoemission with a photon order of up to 9. At a laser intensity of $\sim${}2\ifmmode\times\else\texttimes\fi{}1011\,\,W/cm2 the suppression of the lowest order peak occurs, indicating the onset of strong-field effects. We also observe peak shifting linearly with intensity, with a slope of around -1.0\,\,eV/(1012\,\,W/cm2). We attribute the magnitude of the laser field effects to field enhancement taking place at the tip's surface.
We report on a quantitative measurement of the spatial coherence of electrons emitted from a sharp metal needle tip. We investigate the coherence in photoemission triggered by a near-ultraviolet laser with a photon energy of 3.1 eV and compare it to dc-field emission. A carbon nanotube is brought into close proximity to the emitter tip to act as an electrostatic biprism. From the resulting electron matter wave interference fringes, we deduce an upper limit of the effective source radius both in laser-triggered and dc-field emission mode, which quantifies the spatial coherence of the emitted electron beam. We obtain in laser-triggered and in dc-field emission mode, revealing that the outstanding coherence properties of electron beams from needle tip field emitters are largely maintained in laser-induced emission. In addition, the relative coherence width of 0.36 of the photoemitted electron beam is the largest observed so far. The preservation of electronic coherence during emission as well as ramifications for time-resolved electron imaging techniques are discussed.