In addition to the impact of pollutant emissions, haze pollution is connected with meteorology and climate change. Based on the interannual change analyses of meteorological and environmental observation data from 1981 to 2010, we studied the relationship between the winter haze frequency in central-eastern China (CEC) and the interannual variations of sea surface temperature (SST) over Western Pacific Warm Pool (WPWP) and its underlying mechanism to explore the thermal effect of WPWP on haze pollution variation in China. The results show a significant positive correlation coefficient reaching up to 0.61 between the interannual variations of SST in WPWP and haze pollution frequency in the CEC region over 1981–2010, reflecting the WPWP’s thermal forcing exerting an important impact on haze variation in China. The anomalies of thermal forcing of WPWP could induce to the changes of East Asian winter monsoonal winds and the vertical thermal structures in the troposphere over the CEC region. In the winter with anomalously warm SST over the WPWP, the near-surface winds were declined, and vertical thermal structure in the lower troposphere tended to be stable over the CEC-region, which could be conducive to air pollutant accumulation leading to the more frequent haze occurrences especially the heavy haze regions of Yangtze River Delta (YRD) and Pearl River Delta (PRD); In the winter with the anomalously cold WPWP, it is only the reverse of warm WPWP with the stronger East Asian winter monsoonal winds and the unstable thermal structure in the lower troposphere, which could attribute to the less frequent haze pollution over the CEC region. Our study revealed that the thermal forcing of the WPWP could have a modulation on air environment change in China.
In this study, using the fourth version of the Community Atmosphere Model (CAM4) with a bulk aerosol model parameterization (BAM) for dust size distribution (CAM4-BAM), East Asian dust and its direct radiative feedbacks (DRF) during the Last Glacial Maximum are analyzed by intercomparing results between the experiments with (Active) and without (Passive) the DRF. This CAM4-BAM captures the expected characteristics that the dust aerosol optical depth and loading over East Asia during the Last Glacial Maximum (LGM) were significantly greater compared to the current climate. A comparative analysis of the Active and Passive experiments reveals that consideration of the dust–radiation interaction can significantly reduce dust emissions and then weaken the whole dust cycle, including loading, transport, and dry and wet depositions over East Asia. Further analysis of the dust–radiation feedback shows that the DRF decreases surface sensible heat, mainly owing to the negative surface forcing induced by dust with a value of −11.8 W m−2. The decreased surface sensible heat weakens the turbulent energy within the planetary boundary layer and the surface wind speed, and then reduces the regional dust emissions. This process creates a negative DRF–emission feedback loop to affect the dust cycle during the LGM. Further analysis reveals that the dust emissions in the LGM over East Asia were more reduced, with amounts of −77.2 Tg season−1 by the negative DRF–emission feedback, compared to the current climate with −6.8 Tg season−1. The two ratios of this reduction to their emissions are close to −10.7% for the LGM and −7.5% for the current climate.