This study examines experimentally the hydrodynamic interaction between a regular porous medium and an adjacent free-flow channel at low Reynolds numbers (Re < 1). The porous medium consists of evenly spaced micro-structured rectangular pillars arranged in a uniform pattern, while the free-flow channel features a rectangular cross-sectional area. The overall arrangement comprises a polydimethylsiloxane microfluidic model where distilled water, doped with fluorescent particles, is the examined fluid. Using micro-particle image velocimetry, single-phase quantitative velocity measurements are carried out at the pore scale to reveal the microscopic characteristics of the flow for such a coupled system. Interfacial velocity-slip and stress-jump coefficients are also evaluated with a volume-averaging method based on the Beavers-Joseph and Ochoa-Tapia-Whitaker models, respectively. The results show that, from a microscopic point of view, parallel flow at the interface is not obtained due to the periodically generated U-shaped flow profile between the interface pillars. However, the interface coefficients show no sensitivity to moderate flow angles. The highly resolved experimental information obtained in this study can also be used for the validation of numerical models providing a unique dataset for free-flow and porous media coupled systems.
The mechanism of dynamic wetting and the fluid dynamics during the onset of droplet mobilization driven by a microchannel flow are not clearly understood. In this work, we use microparticle tracking velocimetry to visualize the velocity distribution inside the droplet both prior to and during mobilization. Time-averaged and instantaneous velocity vectors are determined using fluorescent microscopy for various capillary numbers. A circulating flow exists inside the droplet at a subcritical capillary number, in which case the droplet is pinned to the channel walls. When the capillary number exceeds a critical value, droplet mobilization occurs, and this process can be divided into two stages. In the first stage, the location of the internal circulation vortex center moves to the rear of the droplet and the droplet deforms, but the contact lines at the top walls remain fixed. In the second stage, the droplet rolls along the solid wall, with fixed contact angles keeping the vortex center in the rear part of the droplet. The critical capillary number for the droplet mobilization is larger for the droplet fluid with a larger viscosity. A force-balance model of the droplet, considering the effect of fluid properties, is formulated to explain the experimental trends of advancing and receding contact angles with the capillary number. Numerical simulations on internal circulations for the pinned droplet indicate that the reversed flow rate, when normalized by the inlet flow rate and the kinematic viscosity ratio of the wetting and nonwetting phases, is independent of the capillary number and the droplet composition.
15 October 2021 in Journal of Materials Chemistry A
Many engineering technologies such as electronic cooling and thermal desalination exemplify the enhancement of evaporation and boiling heat transfer by surface modification. Nevertheless, the core parameters of heat transfer such as critical heat flux and heat transfer coefficient are associated with surface wettability and morphology. Herein, for the first time, a metal–organic framework (MOF) film, viz. HKUST-1, was integrated into a metallic woven mesh (macroporous support) for enhancing liquid rewetting and capillary-driven evaporation and boiling heat transfer. Compared to bare copper mesh, this architecture was found to significantly increase the critical heat flux by 205% and the heat transfer coefficient by 90%. The complex coupled two-phase (liquid and gas) transport process involving capillary wicking, evaporation, adsorption and desorption were critically examined by analysing the dynamics of multiple interfaces during horizontal wicking. Relying upon visible colorimetric changes, HKUST-1 sustained on the copper woven mesh could expedite quantitative analysis of the coupled capillary evaporation process. In principle, this is primed to offer fundamental insights into the mechanisms of transport phenomena. Introduction of such previously unreported hierarchical porous structures could also potentially advance the state-of-the-art of passive thermal management technologies. In essence, a new route to elicit superhydrophilic surfaces emerges, paving new ways for understanding the intrinsic mechanisms of phase-change heat transfer.