The stratospheric gravity wave field in the Southern Hemisphere is investigated by analyzing observations collected by 27 long-duration balloons that flew between September 2005 and February 2006 over Antarctica and the Southern Ocean. The analysis is based on the methods introduced by Boccara et al. in a companion paper. Special attention is given to deriving information useful to gravity wave drag parameterizations employed in atmospheric general circulation models. The balloon dataset is used to map the geographic variability of gravity wave momentum fluxes in the lower stratosphere. This flux distribution is found to be very heterogeneous with the largest time-averaged value (28 mPa) observed above the Antarctic Peninsula. This value exceeds by a factor of ∼10 the overall mean momentum flux measured during the balloon campaign. Zonal momentum fluxes were predominantly westward, whereas meridional momentum fluxes were equally northward and southward. A local enhancement of southward flux is nevertheless observed above Adélie Land and is attributed to waves generated by katabatic winds, for which the signature is otherwise rather small in the balloon observations. When zonal averages are performed, oceanic momentum fluxes are found to be of similar magnitude to continental values (2.5–3 mPa), stressing the importance of nonorographic gravity waves over oceans. Last, gravity wave intermittency is investigated. Mountain waves appear to be significantly more sporadic than waves observed above the ocean.

In this article, long-duration balloon and spaceborne observations, and mesoscale numerical simulations are used to study the intermittency of gravity waves in the lower stratosphere above Antarctica and the Southern Ocean; namely, the characteristics of the gravity wave momentum-flux probability density functions (pdfs) obtained with these three datasets are described. The pdfs consistently exhibit long tails associated with the occurrence of rare and large-amplitude events. The pdf tails are even longer above mountains than above oceanic areas, which is in agreement with previous studies of gravity wave intermittency in this region. It is moreover found that these rare, large-amplitude events represent the main contribution to the total momentum flux during the winter regime of the stratospheric circulation. In contrast, the wave intermittency significantly decreases when stratospheric easterlies develop in late spring and summer. It is also shown that, except above mountainous areas in winter, the momentum-flux pdfs tend to behave like lognormal distributions. Monte Carlo simulations are undertaken to examine the role played by critical levels in influencing the shape of momentum-flux pdfs. In particular, the study finds that the lognormal shape may result from the propagation of a wave spectrum into a varying background wind field that generates the occurrence of frequent critical levels.

Wave‐induced Lagrangian fluctuations of temperature and vertical velocity in the lower stratosphere are quantified using measurements from superpressure balloons (SPBs). Observations recorded every minute along SPB flights allow the whole gravity wave spectrum to be described and provide unprecedented information on both the intrinsic frequency spectrum and the probability distribution function of wave fluctuations. The data set has been collected during two campaigns coordinated by the French Space Agency in 2010, involving 19 balloons over Antarctica and 3 in the deep tropics. In both regions, the vertical velocity distributions depart significantly from a Gaussian behavior. Knowledge on such wave fluctuations is essential for modeling microphysical processes along Lagrangian trajectories. We propose a new simple parameterization that reproduces both the non‐Gaussian distribution of vertical velocities (or heating/cooling rates) and their observed intrinsic frequency spectrum.

An original and innovative sampling system called AirCore was presented by NOAA in 2010 (Karion et al., 2010). It consists of a long (> 100 m) and narrow (< 1 cm) stainless steel tube that can retain a profile of atmospheric air. The captured air sample has then to be analyzed with a gas analyzer for trace mole fraction. In this study, we introduce a new AirCore aiming to improve resolution along the vertical with the objectives to (i) better capture the vertical distribution of CO₂ and CH₄, (ii) provide a tool to compare AirCores and validate the estimated vertical resolution achieved by AirCores. This (high-resolution) AirCore-HR consists of a 300 m tube, combining 200 m of 0.125 in. (3.175 mm) tube and a 100 m of 0.25 in. (6.35 mm) tube. This new configuration allows us to achieve a vertical resolution of 300 m up to 15 km and better than 500 m up to 22 km (if analysis of the retained sample is performed within 3 h). The AirCore-HR was flown for the first time during the annual StratoScience campaign from CNES in August 2014 from Timmins (Ontario, Canada). High-resolution vertical profiles of CO₂ and CH₄ up to 25 km were successfully retrieved. These profiles revealed well-defined transport structures in the troposphere (also seen in CAMS-ECMWF high-resolution forecasts of CO₂ and CH₄ profiles) and captured the decrease of CO₂ and CH₄ in the stratosphere. The multi-instrument gondola also carried two other low-resolution AirCore-GUF that allowed us to perform direct comparisons and study the underlying processing method used to convert the sample of air to greenhouse gases vertical profiles. In particular, degrading the AirCore-HR derived profiles to the low resolution of AirCore-GUF yields an excellent match between both sets of CH₄ profiles and shows a good consistency in terms of vertical structures. This fully validates the theoretical vertical resolution achievable by AirCores. Concerning CO₂ although a good agreement is found in terms of vertical structure, the comparison between the various AirCores yields a large and variable bias (up to almost 3 ppm in some parts of the profiles). The reasons of this bias, possibly related to the drying agent used to dry the air, are still being investigated. Finally, the uncertainties associated with the measurements are assessed, yielding an average uncertainty below 3 ppb for CH₄ and 0.25 ppm for CO₂ with the major source of uncertainty coming from the potential loss of air sample on the ground and the choice of the starting and ending point of the collected air sample inside the tube. In an ideal case where the sample would be fully retained, it would be possible to know precisely the pressure at which air was sampled last and thus to improve the overall uncertainty to about 0.1 ppm for CO₂ and 2 ppb for CH₄.

The impact of high-frequency fluctuations of temperature on homogeneous nucleation of ice crystals in the vicinity of the tropical tropopause is investigated using a bin microphysics scheme for air parcels. The imposed temperature fluctuations come from measurements during isopycnic balloon flights near the tropical tropopause. The balloons collected data at high frequency, guaranteeing that gravity wave signals are well resolved.With the observed temperature time series, the numerical simulations with homogeneous freezing show a full range of ice number concentration (INC) as previously observed in the tropical upper troposphere. In particular, a low INC may be obtained if the gravity wave perturbations produce a non-persistent cooling rate (even with large magnitude) such that the absolute change in temperature remains small during nucleation. This result is explained analytically by a dependence of the INC on the absolute drop in temperature (and not on the cooling rate). This work suggests that homogeneous ice nucleation is not necessarily inconsistent with observations of low INCs.

Tropical gravity wave activity is investigated using measurements of momentum fluxes gathered during Strateole‐2 superpressure balloon flights. The data set consists of eight balloon flights performed in the deep tropics from November 2019 to February 2020. The flights lasted for 2–3 months each, and in‐situ meteorological data were collected every 30 s. The relation between gravity waves and deep convection is investigated using geostationary satellite data from the NOAA/NCEP GPM_MERGIR satellite data product, at 1 h resolution. The amplitude of gravity wave momentum fluxes shows a clear dependence on the distance to the nearest convective system, with a strong decay as distance to convection increases. The largest momentum‐flux values (>mPa) are only found less than 200 km away from deep convection. The sensitivity of the wave flux to distance from convection is stronger for high frequency gravity waves (periods shorter than 60 min). Lower frequency waves tend to a non‐zero, background value away from convection, supporting some background value in gravity‐wave drag parameterizations. On the other hand, the wide range of momentum flux values observed close to the convection emphasizes the intermittent nature of the gravity‐wave source. The large scale variation of gravity‐wave intermittency within the equatorial belt is also studied. The results highlight spatial variations of gravity wave activity, with the highest momentum flux recorded over land.