High-performance electromagnetic interference shielding is becoming vital for the next generation telecommunication and sensor devices among which portable and wearable applications require highly flexible and lightweight materials having efficient absorption-dominant shielding. Herein, we report on lightweight carbon foam-carbon nanotube/carbon nanofiber nanocomposites that are synthesized in a two-step robust process including a simple carbonization of open-pore structure melamine foams and subsequent growth of carbon nanotubes/nanofibers by chemical vapor deposition. The microstructure of the nanocomposites resemble a 3-dimensional hierarchical network of carbonaceous skeleton surrounded with a tangled web of bamboo-shaped carbon nanotubes and layered graphitic carbon nanofibers. The microstructure of the porous composite enables absorption-dominant (absorbance ~0.9) electromagnetic interference shielding with an effectiveness of ~20-30 dB and with an equivalent mass density normalized shielding effectiveness of ~800-1700 dB cm³ g^-1 at the K-band frequency (18-26.5 GHz). Moreover, the hydrophobic nature of the materials grants water-repellency and stability in humid conditions important for reliable operation in outdoor use; whereas the mechanical flexibility and durability with excellent piezoresistive behavior enable strain-responsive tuning of electrical conductivity and electromagnetic interference shielding, adding on further functionalities. The demonstrated nanocomposites are versatile and will contribute to the development of reliable devices not only in telecommunication but also in wearable electronics, aerospace engineering and robotics among others.

Stretchable and wearable strain sensors have been intensively studied in recent years for applications in human motion monitoring. However, achieving a high-performance strain sensor with high stretchability, ultra-sensitivity, and functionality, such as tunable sensing ranges and sensitivity to various stimuli, has not yet been reported, even though such sensors have great importance for the future applications of wearable electronics. Herein, a novel and versatile strain sensor based on a cracking (silver ink patterned silicone elastomer)-(silver plated nylon structure) (Ag-DS/CF) has been designed and fabricated. The unique structure combined precisely shaped stretchable conductive fabrics and wrinkled Ag-ink pattern to achieve an excellent electrical performance. The Ag-DS/CF could be used to detect both large and subtle human motions and activities, pressure changes, and physical vibrations by achieving high stretchability up to 75%, ultrahigh sensitivity (gauge factor >10⁴–10⁶), tunable sensing ranges (from 7 to 75%). Excellent durability was demonstrated for human motion monitoring with machine washability. The extremely versatile Ag-DS/CF showed outstanding potential for the future of wearable electronics in real-time monitoring of human health, sports performance, etc.

The continuously growing number of short-life electronics equipment inherently results in a massive amount of problematic waste, which poses risks of environmental pollution, endangers human health, and causes socioeconomic problems. Hence, to mitigate these negative impacts, it is our common interest to substitute conventional materials (polymers and metals) used in electronics devices with their environmentally benign renewable counterparts, wherever possible, while considering the aspects of functionality, manufacturability, and cost. To support such an effort, in this study, we explore the use of biodegradable bioplastics, such as polylactic acid (PLA), its blends with polyhydroxybutyrate (PHB) and composites with pyrolyzed lignin (PL), and multiwalled carbon nanotubes (MWCNTs), in conjunction with processes typical in the fabrication of electronics components, including plasma treatment, dip coating, inkjet and screen printing, as well as hot mixing, extrusion, and molding. We show that after a short argon plasma treatment of the surface of hot-blown PLA-PHB blend films, percolating networks of single-walled carbon nanotubes (SWCNTs) having sheet resistance well below 1 kΩ/□ can be deposited by dip coating to make electrode plates of capacitive touch sensors. We also demonstrate that the bioplastic films, as flexible dielectric substrates, are suitable for depositing conductive micropatterns of SWCNTs and Ag (1 kΩ/□ and 1 Ω/□, respectively) by means of inkjet and screen printing, with potential in printed circuit board applications. In addition, we exemplify compounded and molded composites of PLA with PL and MWCNTs as excellent candidates for electromagnetic interference shielding materials in the K-band radio frequencies (18.0–26.5 GHz) with shielding effectiveness of up to 40 and 46 dB, respectively.

The development of flexible and stretchable sensing for future applications, e.g., strain, force, and pressure, requires novel foam and foam-like structures with properties such as fast relaxation times, a wide linear response range, good sensitivity to different stimuli and repeatability, without compromising low-cost, simple and effective manufacturing methods, and excellent mechanical properties. We present a new type of hybrid foam pressure sensor that utilizes a combination of piezoresistive and capacitive sensor elements. The hybrid foam sensor shows a maximum pressure sensitivity of 0.338 kPa ^-1 and a linear response of 0.049 kPa ^- 1 in the piezoresistive and capacitive sensor elements, respectively, in the pressure ranges of <;5 and 0-240 kPa, respectively. The response and recovery times of both sensor elements were similar, ≤200 ms, at various pressures. In addition, the properties of the hybrid foam sensors, e.g., sensitivity and response and recovery times, can be tuned in various ways, such as by changing the thickness of the composition of the foam. In addition, the materials are easily accessible and the sensor can be cost-effectively manufactured and changed for different purposes. The relatively high sensitivity of the piezoresistive sensor element enables object manipulation from low pressure (≥21 Pa) to high pressure (>80 kPa). Simultaneously, both the sensor elements can be used for impact measurements across a wide range of pressures up to ≥240 kPa. Thus, the concept of the hybrid foam sensor could be utilized widely for sensing of pressures, impacts, or even bending in various applications, e.g., wearable electronics.

Ultimately soft electronics seek affordable and high mechanical performance universal self‐healing materials that can autonomously heal in harsh environments within short times scales. As of now, such features are not found in a single material. Herein, interpenetrated elastomer network with bimodal chain length distribution showing rapid autonomous healing in universal conditions (<7200 s) with high efficiency (up to 97.6 ± 4.8%) is reported. The bimodal elastomer displays strain‐induced photoelastic effect and reinforcement which is responsible for its remarkable mechanical robustness (≈5.5 MPa stress at break and toughness ≈30 MJ m⁻³). The entropy‐driven elasticity allows an unprecedented shape recovery efficiency (100%) even after fracturing and 100% resiliency up to its stretching limit (≈2000% strain). The elastomers can be mechanically conditioned leading to a state where they recover their shape extremely quickly after removal of stress (nearly order of magnitude faster than pristine elastomers). As a proof of concept, universal self‐healing mechanochromic strain sensor is developed capable of operating in various environmental conditions and of changing its photonic band gap under mechanical stress.

Fluid balance is important for a healthy human being. In this paper, a method to measure hydration status was developed and tested towards non-invasive measurement from human skin. Measurement of hydration status was performed by a microwave sensor utilizing a complementary split ring resonator (CSRR). The sensor was modeled, manufactured and then characterized by measuring tailor made skin phantoms based on the realistic electrical properties of skin with different degrees of hydration status. Qualitative longer term (>24 h) evaluation of the sensor was also performed by measuring polyester tissue that was drying over the time. Hydration status, represented by dehydrated, normal and hydrated skin phantoms, based on polyurethane with carbon and ceramic additives, was measured successfully by monitoring the changes in resonance frequency around 5.52 GHz. All results were compared to the dielectric reference measurements done by a commercial laboratory instrument.