Tropical tropospheric ozone (TTO) is important for the global radiation budget because the longwave radiative effect of tropospheric ozone is higher in the tropics than midlatitudes. In recent decades the TTO burden has increased, partly due to the ongoing shift of ozone precursor emissions from midlatitude regions toward the Equator. In this study, we assess the distribution and trends of TTO using ozone profiles measured by high-quality in situ instruments from the IAGOS (In-Service Aircraft for a Global Observing System) commercial aircraft, the SHADOZ (Southern Hemisphere ADditional OZonesondes) network, and the ATom (Atmospheric Tomographic Mission) aircraft campaign, as well as six satellite records reporting tropical tropospheric column ozone (TTCO): TROPOspheric Monitoring Instrument (TROPOMI), Ozone Monitoring Instrument (OMI), OMI/Microwave Limb Sounder (MLS), Ozone Mapping Profiler Suite (OMPS)/Modern-Era Retrospective analysis for Research and Applications version 2 (MERRA-2), Cross-track Infrared Sounder (CrIS), and Infrared Atmospheric Sounding Interferometer (IASI)/Global Ozone Monitoring Experiment 2 (GOME2). With greater availability of ozone profiles across the tropics we can now demonstrate that tropical India is among the most polluted regions (e.g., western Africa, tropical South Atlantic, Southeast Asia, Malaysia and Indonesia), with present-day 95th percentile ozone values reaching 80 nmol mol⁻¹ in the lower free troposphere, comparable to midlatitude regions such as northeastern China and Korea. In situ observations show that TTO increased between 1994 and 2019, with the largest mid- and upper-tropospheric increases above India, Southeast Asia, and Malaysia and Indonesia (from 3.4 ± 0.8 to 6.8 ± 1.8 nmol mol⁻¹ decade⁻¹), reaching 11 ± 2.4 and 8 ± 0.8 nmol mol⁻¹ decade⁻¹ close to the surface (India and Malaysia–Indonesia, respectively). The longest continuous satellite records only span 2004–2019 but also show increasing ozone across the tropics when their full sampling is considered, with maximum trends over Southeast Asia of 2.31 ± 1.34 nmol mol⁻¹ decade⁻¹ (OMI) and 1.69 ± 0.89 nmol mol⁻¹ decade⁻¹ (OMI/MLS). In general, the sparsely sampled aircraft and ozonesonde records do not detect the 2004–2019 ozone increase, which could be due to the genuine trends on this timescale being masked by the additional uncertainty resulting from sparse sampling. The fact that the sign of the trends detected with satellite records changes above three IAGOS regions, when their sampling frequency is limited to that of the in situ observations, demonstrates the limitations of sparse in situ sampling strategies. This study exposes the need to maintain and develop high-frequency continuous observations (in situ and remote sensing) above the tropical Pacific Ocean, the Indian Ocean, western Africa, and South Asia in order to estimate accurate and precise ozone trends for these regions. In contrast, Southeast Asia and Malaysia–Indonesia are regions with such strong increases in ozone that the current in situ sampling frequency is adequate to detect the trends on a relatively short 15-year timescale.

The Community Long-term Infrared Microwave Combined Atmospheric Product System (CLIMCAPS) retrieves vertical profiles of temperature, water vapor, greenhouse and pollutant gases, and cloud properties from measurements made by infrared and microwave instruments on polar-orbiting satellites. These are AIRS/AMSU on Aqua and CrIS/ATMS on Suomi NPP and NOAA20; together they span nearly 2 decades of daily observations (2002 to present) that can help characterize diurnal and seasonal atmospheric processes from different time periods or regions across the globe. While the measurements are consistent, their information content varies due to uncertainty stemming from (i) the observing system (e.g., instrument type and noise, choice of inversion method, algorithmic implementation, and assumptions) and (ii) localized conditions (e.g., presence of clouds, rate of temperature change with pressure, amount of water vapor, and surface type). CLIMCAPS quantifies, propagates, and reports all known sources of uncertainty as thoroughly as possible so that its retrieval products have value in climate science and applications. In this paper we characterize the CLIMCAPS version 2.0 system and diagnose its observing capability (ability to retrieve information accurately and consistently over time and space) for seven atmospheric variables – temperature, H₂O, CO, O₃, CO₂, HNO₃, and CH₄ – from two satellite platforms, Aqua and NOAA20. We illustrate how CLIMCAPS observing capability varies spatially, from scene to scene, and latitudinally across the globe. We conclude with a discussion of how CLIMCAPS uncertainty metrics can be used in diagnosing its retrievals to promote understanding of the observing system and the atmosphere it measures.

The Community Long-term Infrared Microwave Combined Atmospheric Product System (CLIMCAPS) retrieves multiple Essential Climate Variables (ECV) about the vertical atmosphere from hyperspectral infrared measurements made by the Atmospheric InfraRed Sounder (AIRS, 2002–present) and its successor, the Cross-track Infrared Sounder (CrIS, 2011–present). CLIMCAPS ECVs are profiles of temperature and water vapor, column amounts of greenhouse gases (CO₂, CH₄), ozone (O₃) and precursor gases (CO, SO₂) as well as cloud properties. AIRS (and CrIS) spectral measurements are highly correlated signals of many atmospheric state variables. CLIMCAPS inverts an AIRS (and CrIS) measurement into a set of discrete ECVs by employing a sequential Bayesian approach in which scene-dependent uncertainty is rigorously propagated. This not only linearizes the inversion problem but explicitly accounts for spectral interference from other state variables so that the correlation among ECVs (and their uncertainty) may be minimized. Here, we outline the CLIMCAPS retrieval methodology with specific focus given to its sequential scene-dependent uncertainty propagation system. We conclude by demonstrating continuity in two CLIMCAPS ECVs across AIRS and CrIS so that a long-term data record may be generated to study the feedback cycles characterizing our climate system.

The dual‐regression (DR) method retrieves information about the Earth surface and vertical atmospheric conditions from measurements made by any high‐spectral resolution infrared sounder in space. The retrieved information includes temperature and atmospheric gases (such as water vapor, ozone, and carbon species) as well as surface and cloud top parameters. The algorithm was designed to produce a high‐quality product with low latency and has been demonstrated to yield accurate results in real‐time environments. The speed of the retrieval is achieved through linear regression, while accuracy is achieved through a series of classification schemes and decision‐making steps. These steps are necessary to account for the nonlinearity of hyperspectral retrievals. In this work, we detail the key steps that have been developed in the DR method to advance accuracy in the retrieval of nonlinear parameters, specifically cloud top pressure. The steps and their impact on retrieval results are discussed in‐depth and illustrated through relevant case studies. In addition to discussing and demonstrating advances made in addressing nonlinearity in a linear geophysical retrieval method, advances toward multi‐instrument geophysical analysis by applying the DR to three different operational sounders in polar orbit are also noted. For any area on the globe, the DR method achieves consistent accuracy and precision, making it potentially very valuable to both the meteorological and environmental user communities.

Satellite meteorology is a relatively new branch of the atmospheric sciences. The field emerged in the late 1950s during the Cold War and built on the advances in rocketry after World War II. In less than 70 years, satellite observations have transformed the way scientists observe and study Earth. This paper discusses some of the key advances in our understanding of the energy and water cycles, weather forecasting, and atmospheric composition enabled by satellite observations. While progress truly has been an international achievement, in accord with a monograph observing the centennial of the American Meteorological Society, as well as limited space, the emphasis of this chapter is on the U.S. satellite effort.

In this paper, we describe how researchers and weather forecasters work together to make satellite sounding data sets more useful in severe weather forecasting applications through participation in National Oceanic and Atmospheric Administration (NOAA)’s Hazardous Weather Testbed (HWT) and JPSS Proving Ground and Risk Reduction (PGRR) program. The HWT provides a forum for collaboration to improve products ahead of widespread operational deployment. We found that the utilization of the NOAA-Unique Combined Atmospheric Processing System (NUCAPS) soundings was improved when the product developer and forecaster directly communicated to overcome misunderstandings and to refine user requirements. Here we share our adaptive strategy for (1) assessing when and where NUCAPS soundings improved operational forecasts by using real, convective case studies and (2) working to increase NUCAPS utilization by improving existing products through direct, face-to-face interaction. Our goal is to discuss the lessons we learned and to share both our successes and challenges working with the weather forecasting community in designing, refining, and promoting novel products. We foresee that our experience in the NUCAPS product development life cycle may be relevant to other communities who can then build on these strategies to transition their products from research to operations (and operations back to research) within the satellite meteorological community.