High-quality densely packed hexagonal arrays of Ni nanowires have been prepared by filling self-ordered nanopores in alumina membranes. Nanowires with different diameter d (18–83 nm) and lattice parameter D (65 and 105 nm) have been studied by atomic force, high resolution scanning electron microscopies, Rutherford backscattering, and vibrating sample magnetometer techniques. Axial loops coercivity and remanence decrease with increasing ratio diameter to lattice parameter, r, until nanowires start to interconnect locally. Additionally, hysteresis of in-plane loops increases with packing factor. In order to interpret the experimental results, multipolar magnetostatic interactions among nanowires with increasing ratio r are considered.

The exchange bias of antiferromagnetic-ferromagnetic (AFM-FM) bilayers is found to be strongly dependent on the ferromagnetic spin configuration. The widely accepted inverse proportionality of the exchange bias field with the ferromagnetic thickness is broken in FM layers thinner than the FM correlation length. Moreover, an anomalous thermal dependence of both exchange bias field and coercivity is also found. A model based on springlike domain walls parallel to the AFM-FM interface quantitatively accounts for the experimental results and, in particular, for the deviation from the inverse proportionality law. These results reveal the active role the ferromagnetic spin structure plays in AFM-FM hybrids which leads to a new paradigm of the exchange bias phenomenon.

We report on the magneto-optical properties of hexagonally arranged Ni nanowires embedded in anodic alumina templates. Due to the nanowire geometry, these samples show different response depending on the polarization orientation of the incident light, which leads to a high anisotropy of both their optical and magneto-optical properties. A strong increase of the magneto-optical activity is clearly observed with respect to the Ni bulk material. We associate this behavior to plasmon resonance of the Ni nanowires.

The influence of the macroscopic size of the Ni nanowire array system on their remanence state has been investigated. A simple magnetic phenomenological model has been developed to obtain the remanence as a function of the magnetostatic interactions in the array. We observe that, due to the long range of the dipolar interactions between the wires, the size of the sample strongly influence the remanence of the array. On the other hand, the magnetic state of nanowires has been studied by variable field magnetic force microscopy for different remanent states. The distribution of nanowires with the magnetization in up or down directions and the subsequent remanent magnetization has been deduced from the magnetic images. The existence of two short-range magnetic orderings with similar energies can explain the typical labyrinth pattern observed in magnetic force microscopy images of the nanowire arrays.