The generation of ultrahigh intensity laser pulses was investigated by tightly focusing a wavefront-corrected multi-petawatt Ti:sapphire laser. For the wavefront correction of the PW laser, two stages of deformable mirrors were employed. The multi-PW laser beam was tightly focused by an f/1.6 off-axis parabolic mirror and the focal spot profile was measured. After the wavefront correction, the Strehl ratio was about 0.4, and the spot size in full width at half maximum was 1.5×1.8 μm², close to the diffraction-limited value. The measured peak intensity was 5.5×10²² W/cm², achieving the highest laser intensity ever reached.

Brightness of high-order harmonics is optimized in the space domain by profile flattening and self-guiding of intense femtosecond laser pulse and in the time domain by controlling the laser chirp. The profile flattening and self-guiding of the laser pulse propagating through a long gas jet effectively increased the phase-matched harmonic generation volume, thereby obtaining strong harmonics with low beam divergence, and the laser chirp control allowed the generation of spectrally sharp harmonics. At optimized conditions, the $61\text{st}$ harmonic, obtained at $134\mathrm{\AA }$ from Ne, had a brightness of about $1\times {10}^{15}\mathrm{W}∕{\text{cm}}^2∕\text{srad}$ with a beam divergence of 0.5 mrad and a spectral bandwidth of $0.7\mathrm{\AA }$.

High-harmonic radiation emitted from molecules in a strong laser field contains information on molecular structure and dynamics. When multiple molecular orbitals participate in high-harmonic generation, resolving the contribution of each orbital is crucial for understanding molecular dynamics and for extending high-harmonic spectroscopy to more complicated molecules. We show that two-dimensional high-harmonic spectroscopy can resolve high-harmonic radiation emitted from the two highest-occupied molecular orbitals, HOMO and HOMO-1, of aligned molecules. By the application of an orthogonally polarized two-color laser field that consists of the fundamental and its second-harmonic fields to aligned ${\mathrm{CO}}_2$ molecules, the characteristics attributed to the two orbitals are found to be separately imprinted in odd and even harmonics. Two-dimensional high-harmonic spectroscopy may open a new route to investigate ultrafast molecular dynamics during chemical processes.

Laser wakefield electron acceleration (LWFA) is an emerging technology for the next generation of electron accelerators. As intense laser technology has rapidly developed, LWFA has overcome its limitations and has proven its possibilities to facilitate compact high-energy electron beams. Since high-power lasers reach peak power beyond petawatts (PW), LWFA has a new chance to explore the multi-GeV energy regime. In this article, we review the recent development of multi-GeV electron acceleration with PW lasers and discuss the limitations and perspectives of the LWFA with high-power lasers.

We propose a novel injection scheme for laser-driven wakefield acceleration in which controllable localized electron injection is obtained by inserting nanoparticles into a plasma medium. The nanoparticles provide a very confined electric field that triggers localized electron injection where nonlinear plasma waves are excited but not sufficient for background electrons self-injection. We present a theoretical model to describe the conditions and properties of the electron injection in the presence of nanoparticles. Multi-dimensional particle-in-cell (PIC) simulations demonstrate that the total charge of the injected electron beam can be controlled by the position, number, size, and density of the nanoparticles. The PIC simulation also indicates that a 5-GeV electron beam with an energy spread below 1% can be obtained with a 0.5-PW laser pulse by using the nanoparticle-assisted laser wakefield acceleration.

We report here a systematic quantitative study on the generation and characteristics of an active muon source driven by the interaction of an electron beam within the energy range of 1–10 GeV from laser wakefield acceleration (LWFA) with a tungsten target, using Monte Carlo simulations. The 10 GeV electron beam, achievable in the near future, from LWFA using femtosecond multi-PW lasers is employed to drive the bright source of muon pairs in a compact setup. We show that a highly directional and intense source of short-pulsed GeV muon pairs ( μ ⁻ μ ⁺ ) have a peak brightness of 5 × 10 ¹⁷ pairs s ^–1 cm ^–2 sr ^–1 and sub-100 ps duration could be produced using a quasi-monoenergetic 10 fs, 10 GeV electron bunch with a 1-mrad divergence and 100 pC charge. The muon pairs are emitted from a point-like source with a well-defined position and timing; the source has a size and geometric emittance of about 1 mm and 40 μ m, respectively. Such muon sources can greatly benefit applications in muon radiography as well as studies on anomalous dipole moments, rare decays of muons, neutrino oscillations, and an injector for a future compact muon collider.