The efficient interaction of light with quantum emitters is crucial to most applications in nano and quantum photonics, such as sensing or quantum information processing. Effective excitation and photon extraction are particularly important for the weak signals emitted by a single atom or molecule. Recent works have introduced novel collection strategies, which demonstrate that large efficiencies can be achieved by either planar dielectric antennas combined with high numerical aperture objectives or optical nanostructures that beam emission into a narrow angular distribution. However, the first approach requires the use of elaborate collection optics, while the latter is based on accurate positioning of the quantum emitter near complex nanoscale architectures; hence, sophisticated fabrication and experimental capabilities are needed. Here we present a theoretical and experimental demonstration of a planar optical antenna that beams light emitted by a single molecule, which results in increased collection efficiency at small angles without stringent requirements on the emitter position. The proposed device exhibits broadband performance and is spectrally scalable, and it is simple to fabricate and therefore applies to a wide range of quantum emitters. Our design finds immediate application in spectroscopy, quantum optics and sensing.
6 January 2011 in Solar Energy Materials and Solar Cells
The purpose of this work is to understand the fundamental connection between structural correlations and light localization in three-dimensional (3D) open scattering systems of finite size. We numerically investigate the transport of vector electromagnetic waves scattered by resonant electric dipoles spatially arranged in 3D space by stealthy hyperuniform disordered point patterns. Three-dimensional stealthy hyperuniform disordered systems are engineered with different structural correlation properties determined by their degree of stealthiness . Such fine control of exotic states of amorphous matter enables the systematic design of optical media that interpolate in a tunable fashion between uncorrelated random structures and crystalline materials. By solving the electromagnetic multiple scattering problem using Green's matrix spectral method, we establish a transport phase diagram that demonstrates a distinctive transition from a diffusive to a weak localization regime beyond a critical scattering density that depends on . The transition is characterized by studying the Thouless number and the spectral statistics of the scattering resonances. In particular, by tuning the parameter, we demonstrate large spectral gaps and suppressed subradiant proximity resonances, facilitating light localization. Moreover, consistently with previous studies, our results show a region of the transport phase diagram where the investigated scattering systems become transparent. Our work provides a systematic description of the transport and weak localization properties of light in stealthy hyperuniform structures and motivates the engineering of photonic systems with enhanced light-matter interactions for applications to both classical and quantum devices.
By using the dyadic Green's matrix spectral method, we demonstrate that aperiodic deterministic Vogel spirals made of electric dipoles support a light localization transition in three dimensions, an effect that does not occur in traditional uniform random media. We discover a light localization transition in Vogel spiral arrays embedded in three-dimensional space by evaluating the Thouless conductance, the level spacing statistics, and by performing a finite-size scaling. We probe light localization in the plane of the array by analyzing the behavior of the scattering resonances in three-dimensional space. This light localization transition is different from the Anderson transition because Vogel spirals are aperiodic deterministic structures characterized by nonuniform geometries. Moreover, this transition occurs when the vector character of light is fully taken into account, in contrast to what is expected for traditional uniform random media of pointlike scatterers. We show that light localization in Vogel arrays is a collective phenomenon that involves the contribution of multiple length scales. Vogel spirals are suitable photonic platforms to localize light thanks to their distinctive structural correlation properties that enable collective electromagnetic excitations with strong light-matter coupling. Our results unveil the importance of aperiodic correlations for the engineering of photonic media with strongly enhanced light-matter coupling compared to the traditional periodic and homogeneous random media.
A transfer matrix model of a luminescent down-shifter (LDS) layer, consisting of silicon nanocrystals (Si-NCs) embedded in a silicon oxide matrix, on a silicon solar cells is presented. To enhance the efficiency of the silicon solar cell, we propose using a SiO2/Si-NCs double layer stack, as an anti-reflection-coating (ARC) and as a LDS material. The optical characteristics of this stack have been simulated and optimized as a front surface coating. The cell performances have been simulated by means of a two-dimensional device simulator and compared with the performances of a reference silicon solar cell. We found a 6% relative enhancement of the energy conversion efficiency with respect to the reference cell. We demonstrate that this enhancement results from the lower reflectance and from the down-shifter effect of the Si-NCs activated coating stack.