We report on a new random laser phenomenon that gives rise to narrow emission modes without requiring optical cavities. Sharp emission peaks are observed experimentally over a broad range of scattering strengths and analyzed in numerical calculations. We find that the introduction of exponential gain in a multiple light scattering process strongly increases the importance of very long light paths. Such long paths are rare and often neglected in passive disordered materials but we show that they can dominate the emission spectrum from an amplifying disordered system.
A novel one-step in situ synthesis of gold nanostars (AuNSs) on a pre-cured polydimethylsiloxane (PDMS) film is proposed for the fabrication of highly sensitive surface-enhanced Raman scattering (SERS) substrates. Plasmonic activity of the substrates was investigated by collecting SERS maps of 4-mercaptobenzoic acid (4-MBA). The applicability of these flexible substrates is further demonstrated by SERS-based pesticide detection on fruit skin.
A simple and fast one-step fabrication method of silver nanoparticles (AgNPs) on a polydimethylsiloxane (PDMS) film and their improvement as highly sensitive surface enhanced Raman scattering (SERS) substrates via atomically thin Au coatings is demonstrated. The thin Au layer provides oxidation resistivity while maintaining the broad spectral range SERS sensitivity of Ag nanoparticles.