The essential information required for the analysis of Raman lidar water vapor and aerosol data acquired by use of a single laser wavelength is compiled here and in a companion paper [Appl. Opt. 42, 2593 (2003)]. Various details concerning the evaluation of the lidar equations when Raman scattering is measured are covered. These details include the influence of the temperature dependence of both pure rotational and vibrational-rotational Raman scattering on the lidar profile. The full temperature dependence of the Rayleigh-Mie and Raman lidar equations are evaluated by use of a new form of the lidar equation where all the temperature dependence is carried in a single term. The results indicate that, for the range of temperatures encountered in the troposphere, the magnitude of the temperature-dependent effect can reach 10% or more for narrowband Raman water-vapor measurements. Also, the calculation of atmospheric transmission, including the effects of depolarization, is examined carefully. Various formulations of Rayleigh cross-section determination commonly used in the lidar field are compared and reveal differences of as much as 5% among the formulations. The influence of multiple scattering on the measurement of aerosol extinction with the Raman lidar technique is considered, as are several photon pulse pileup-correction techniques.

In a companion paper [Appl. Opt. 42, 2571 (2003)] the temperature dependence of Raman scattering and its influence on the Raman and Rayleigh-Mie lidar equations were examined. New forms of the lidar equation were developed to account for this temperature sensitivity. Here those results are used to derive the temperature-dependent forms of the equations for the water-vapor mixing ratio, the aerosol scattering ratio, the aerosol backscatter coefficient, and the extinction-to-backscatter ratio. The error equations are developed, the influence of differential transmission is studied, and several laser sources are considered in the analysis. The results indicate that the temperature functions become significant when narrowband detection is used. Errors of 5% and more can be introduced into the water-vapor mixing ratio calculation at high altitudes, and errors larger than 10% are possible for calculations of aerosol scattering ratio and thus of aerosol backscatter coefficient and of extinction-to-backscatter ratio.

The NASA Goddard Space Flight Center (GSFC) Scanning Raman Lidar (SRL) participated in the International H2O Project (IHOP), which occurred in May and June 2002 in the midwestern part of the United States. The SRL received extensive optical modifications prior to and during the IHOP campaign that added new measurement capabilities and enabled unprecedented daytime water vapor measurements by a Raman lidar system. Improvements were also realized in nighttime upper-tropospheric water vapor measurements. The other new measurements that were added to the SRL for the IHOP deployment included rotational Raman temperature, depolarization, cloud liquid water, and cirrus cloud ice water content. In this first of two parts, the details of the operational configuration of the SRL during IHOP are provided along with a description of the analysis and calibration procedures for water vapor mixing ratio, aerosol depolarization, and cirrus cloud extinction-to-backscatter ratio. For the first time, a Raman water vapor lidar calibration is performed, taking full account of the temperature sensitivity of water vapor and nitrogen Raman scattering. Part II presents case studies that permit the daytime and nighttime error statistics to be quantified.

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A high-performance Raman lidar operating in the UV portion of the spectrum has been used to acquire, for the first time using a single lidar, simultaneous airborne profiles of the water vapor mixing ratio, aerosol backscatter, aerosol extinction, aerosol depolarization and research mode measurements of cloud liquid water, cloud droplet radius, and number density. The Raman Airborne Spectroscopic Lidar (RASL) system was installed in a Beechcraft King Air B200 aircraft and was flown over the mid-Atlantic United States during July–August 2007 at altitudes ranging between 5 and 8 km. During these flights, despite suboptimal laser performance and subaperture use of the telescope, all RASL measurement expectations were met, except that of aerosol extinction. Following the Water Vapor Validation Experiment—Satellite/Sondes (WAVES_2007) field campaign in the summer of 2007, RASL was installed in a mobile trailer for ground-based use during the Measurements of Humidity and Validation Experiment (MOHAVE-II) field campaign held during October 2007 at the Jet Propulsion Laboratory’s Table Mountain Facility in southern California. This ground-based configuration of the lidar hardware is called Atmospheric Lidar for Validation, Interagency Collaboration and Education (ALVICE). During the MOHAVE-II field campaign, during which only nighttime measurements were made, ALVICE demonstrated significant sensitivity to lower-stratospheric water vapor. Numerical simulation and comparisons with a cryogenic frost-point hygrometer are used to demonstrate that a system with the performance characteristics of RASL–ALVICE should indeed be able to quantify water vapor well into the lower stratosphere with extended averaging from an elevated location like Table Mountain. The same design considerations that optimize Raman lidar for airborne use on a small research aircraft are, therefore, shown to yield significant dividends in the quantification of lower-stratospheric water vapor. The MOHAVE-II measurements, along with numerical simulation, were used to determine that the likely reason for the suboptimal airborne aerosol extinction performance during the WAVES_2007 campaign was a misaligned interference filter. With full laser power and a properly tuned interference filter, RASL is shown to be capable of measuring the main water vapor and aerosol parameters with temporal resolutions of between 2 and 45 s and spatial resolutions ranging from 30 to 330 m from a flight altitude of 8 km with precision of generally less than 10%, providing performance that is competitive with some airborne Differential Absorption Lidar (DIAL) water vapor and High Spectral Resolution Lidar (HSRL) aerosol instruments. The use of diode-pumped laser technology would improve the performance of an airborne Raman lidar and permit additional instrumentation to be carried on board a small research aircraft. The combined airborne and ground-based measurements presented here demonstrate a level of versatility in Raman lidar that may be impossible to duplicate with any other single lidar technique.

The NASA GSFC Scanning Raman Lidar (SRL) participated in the International H2O Project (IHOP) that occurred in May and June 2002 in the midwestern part of the United States. The SRL system configuration and methods of data analysis were described in Part I of this paper. In this second part, comparisons of SRL water vapor measurements and those of Lidar Atmospheric Sensing Experiment (LASE) airborne water vapor lidar and chilled-mirror radiosonde are performed. Two case studies are then presented: one for daytime and one for nighttime. The daytime case study is of a convectively driven boundary layer event and is used to characterize the daytime SRL water vapor random error characteristics. The nighttime case study is of a thunderstorm-generated cirrus cloud case that is studied in its meteorological context. Upper-tropospheric humidification due to precipitation from the cirrus cloud is quantified as is the cirrus cloud optical depth, extinction-to-backscatter ratio, ice water content, cirrus particle size, and both particle and volume depolarization ratios. A stability and back-trajectory analysis is performed to study the origin of wave activity in one of the cloud layers. These unprecedented cirrus cloud measurements are being used in a cirrus cloud modeling study.