Aerosol–planetary boundary layer (PBL) interaction has been proposed as a key mechanism for stabilizing the atmosphere and exacerbating surface air pollution. Although the understanding of this process has progressed enormously, its magnitude and impact remain uncertain and vary widely concerning aerosol types, vertical distributions, synoptic conditions, etc. In this study, our primary interest is to distinguish the aerosol–PBL interaction of absorbing and scattering aerosols under contrasting synoptic patterns and aerosol vertical distributions. Detailed in situ aircraft (King Air 350) measurements and online coupled model Weather Research and Forecasting with Chemistry (WRF-Chem) simulations are explored over the North China Plain (NCP). Furthermore, a long-term PBL stability trend from 1980 to 2020 over the NCP is also investigated. The aircraft measurements and surface observations show that the surface air pollution over the city of Baoding on 3 January is heavier than that on 4 January 2020. In addition, the aerosols are restricted to the low layer on 3 January, whereas the aerosols mix more homogeneously in an upwards direction on 4 January. Thus, we focus on the 2 d with distinct synoptic circumstances, PBL stability, and aerosol vertical distributions over the NCP. According to the WRF-Chem modeling, the synoptic pattern over Baoding differs between the 2 d. The prevailing wind direction is opposite with a southwesterly wind on 3 January and a northeasterly wind on 4 January. The results indicate that the synoptic condition may affect the PBL thermal structure, thus affecting the aerosol vertical distribution. Additionally, the sensitive numerical experiments reveal that the light-absorbing and light-scattering aerosols have different effects on altering the PBL thermal structure. The inhibition effect of scattering aerosols on the PBL appears to be independent of the aerosol height distribution and solely depends on its concentration. However, the aerosol–PBL feedback of absorbing aerosols is highly dependent on its vertical distribution. Besides the 2 d case investigation, the analysis of the modeling results for nearly 1 month from 3 to 30 January 2020 in Baoding yields a more robust and representative conclusion. Our analysis highlights that we should principally concentrate on controlling the emissions of scattering aerosols under the stable stratification, while cooperating to control the emissions of scattering and absorbing aerosols in an unstable stratification. Moreover, the long-term interannual variation in the PBL stability shows a strong correlation with the East Asian winter monsoon, which seems to be valuable in determining which pollutants to target in different monsoon years and attaining more precise air pollution control. Based on the numerical simulations and observational constraints, a concept scheme description has been concluded to deepen our recognition of the interactions between thermodynamic stability and aerosols within the PBL over the NCP region.

Synthesis of uniform and dense metal nanostructures on the whole exposed fiber, instead of simply on the membrane surface, is necessary for controllable separation and sensitive SERS detection. Herein, uniform and dense AuNP/MoS₂ hybrids were synthesized on single 3D glass fiber (GF) surfaces, obtained by the reaction of a MoS₂ nanosheet and HAuCl₄. The chemical mechanism (CM) of the MoS₂ layers and the electromagnetic enhancement (EM) of the dense AuNPs were used to enhance the SERS sensitivity. The molecule-separation ability of the obtained GF membranes, constructed by numerous compacted fibers with dense AuNP/MoS₂ hybrids, was not destroyed, and herein, these membranes were used to separate mixed molecules. These MoS₂-based hybrid substrates show great potential for excellent paper-based separation and are sensitive SERS substrates for biological and chemical detection.

Due to the space and time constraints of turbulence measurement equipment and the experiment scene, it is difficult to obtain the atmosphere refractive index structure constant over the ocean. In this paper, the characteristics of atmospheric optical turbulence in offshore and open ocean conditions are summarized by analyzing the meteorological data obtained from two ocean atmospheric optical parameter field experiments. Because of the influence of land undersurface, the turbulence strength in offshore conditions is roughly the same as that on land and presents different characteristics in open ocean. Compared with the offshore area, the turbulence strength over the open ocean near-surface decreases during the day and increases at night, and the diurnal variation characteristics weaken. The turbulence strength profiles over the offshore area show different characteristics at different times, where the turbulence strength in the morning is higher than that in the evening. By retrieving the meteorological factors affecting the turbulence, it is found that the temperature gradient and wind shear are in good agreement with turbulence strength in both offshore and open ocean areas. Furthermore, the integrated parameters for astronomy and optical telecommunication are derived from profiles over the offshore and open ocean areas. It is of great significance to research the turbulent characteristics of ocean atmosphere for optical transmission and astronomical observations.

The analytical expression of the cross-spectral density function of a twisted anisotropic Gaussian Schell-model (TAGSM) beam transmitting in turbulent ocean is derived by applying a tensor method. The statistical properties, including spectral density, the strength of twist and beam width of the propagating beam are studied carefully through numerical examples. It is demonstrated that the turbulence of ocean has no effect on the rotation direction of the beam spot during propagation. However, the beam shape will degrade into a Gaussian profile under the action of oceanic turbulence with sufficiently long propagation distance, and a beam with a larger initial twist factor is more resistant to turbulence-induced degeneration. As oceanic turbulence becomes stronger, the beam spot spreads more quickly while the twist factor drops more rapidly upon propagation. The physical mechanisms of these phenomena are addressed in detail. The obtained results will be helpful in optical communication systems underwater.

Abstract We firstly propose a roadmap for the design of high repetition rate (~100 MHz) Tm-doped ultrafast fiber laser with an emission wavelength above 2000 nm. This roadmap is confirmed by both theoretical simulation and experimental verification. The designed Tm-doped fiber oscillator not only operates in continuous wave regime with a broad tunable wavelength range of ~ 100 nm, but also in mode-locking regime with an emission wavelength > 2000 nm (up to 2020 nm). A 470-fs laser pulse with a pulse repetition rate of ~96 MHz and the maximum average power of 50 mW are achieved at the output wavelength of 2007 nm, matching well with the theoretical prediction. In a further step, the seed laser pulse is amplified to 3.3 W, accompanied by a Raman frequency shift of the output wavelength to 2346 nm. The homogeneous intense broadband spectrum with a bandwidth of 240-nm centered at 2200 nm is also observed.

Temperature inversion plays an important role in the accumulation and diffusion of aerosols. In this study, the relationship between temperature inversion and the vertical distribution of aerosols is investigated based on Raman lidar observations taken from January 2010 to September 2015 at the Atmospheric Radiation Measurement site in the Southern Great Plains, USA. First, the diurnal and seasonal variations of the surface-based inversion (SBI) and elevated temperature inversion (EI) are investigated. The results indicate that the occurrence frequency of SBI and EI have different seasonal trends. SBI has the highest frequency in summer, while EI has the highest frequency in winter. The diurnal variation of SBI is obvious, with a higher frequency in nighttime and a lower frequency in daytime. The inversion intensity (ΔT) and inversion depth (ΔZ) of SBI and EI have consistent diurnal and seasonal trends. The effects of SBI and EI on the vertical distribution of aerosols are then analyzed. The mean aerosol optical depth (AOD) below the SBI height shows a clear seasonal variation, which is consistent with the seasonal trends of ΔT and ΔZ. This phenomenon also occurs on the AOD below EI top height. The sensitivity analysis shows that the mean AOD below SBI height or EI top height increases with an increase of the ΔT and ΔZ of SBI (EI). It indicates that ΔT and ΔZ are the key factors affecting the vertical distribution of aerosols. In addition, the variation of AOD below and above EI top height is opposite to that of AOD below and above EI bottom height under different ΔT and ΔZ conditions. The correlation coefficients between ΔT (ΔZ) of EI with AOD in EI were 0.62 (0.65). These results indicate that the space between EI bottom height and EI top height can store aerosols. The larger the ΔZ of EI, the more aerosols are stored. These findings contribute to our understanding of the effect of temperature inversion on the vertical distribution of aerosols.