We use inelastic neutron scattering to establish the modulation vectors δ and correlation lengths for the incommensurate magnetic fluctuations in metallic samples of with x=0.075 and 0.14. In notation appropriate for a square lattice where the magnetic instability in the undoped case occurs at (π,π), the vectors δ are along (π,0) and (0,π). The correlation length ξ is larger than the distance between carriers, is weakly dependent on x, and changes significantly between 12 and 100 K for both compositions.
13 May 1991 in Journal of Physics: Condensed Matter
The magnetic structures of the hexagonal and oxides (space group have been studied by neutron-diffraction experiments on powder samples. This study has been complemented with magnetic susceptibility and specific-heat measurements. They confirm that and become ordered below K and K, respectively, according to a triangular antiferromagnetic structure. The latter compound undergoes a second magnetic transition below 75 K, corresponding to a spin reorientation. The presence of weak ferromagnetism of Dzialoshinskii-Moriya type is observed in all the ordered region for the Sc material. In both compounds the moments are contained in the plane and oriented perpendicular or parallel to the [100] directions. The low-temperature ordered moments are and at K. The different behavior observed in the thermal evolution of the magnetic structure of both compounds is discussed in terms of geometrical parameters determined from high-resolution structural data. The origin of the weak ferromagnetism in is also analyzed.
We search for general patterns that explain the low field magnetoresistance at low temperatures in the system . The observed linear dependence of the low field magnetoresistance with the saturation magnetization for the series is related to the antisite disorder at the and sites. This is explained in terms of a spin dependent crossing of intragranular barriers originated from the presence of antiferromagnetic patches that naturally develop when antisite disorder occurs in the double perovskite. The presence of a moderate level of antisite disorder is at the very root of low field magnetoresistance although effects such as disorder distribution, connectivity, or morphology add their contribution.