The significant differences in the activities of 210Pb, 210Bi, 210Po and cosmogenic 7Be and 22Na radionuclides in the urban aerosol samples collected in the summers 2010 and 2011 in the Lodz city of Poland were observed. Simultaneous measurement of these radionuclides, after a simple modification of the one compartment model, allows us to calculate both: the corrected aerosol residence times in the troposphere (1 ÷ 25 days) and in the lower stratosphere (103 ÷ 205 days). The relative input of the additional sources (beside of the 222Rn decay in the air) to the total activity concentrations of 210Pb, 210Bi and 210Po radionuclides in the urban air, plays a substantial role (up to 97% of the total activity) only in the case of 210Po.
3 December 2009 in Journal of Radioanalytical and Nuclear Chemistry
Low-energy X and γ radiations (for example of 210Pb: Eγ = 46.5 keV) are effectively self-absorbed even in thin environmental samples, including air filters with captured dust or contaminated soil, as well as in bottom sediment matrixes with limited quantities of the samples. In this paper, a simple method for the direct analysis of 210Pb (T1/2 = 22.3 years) by gamma-ray spectrometry in environmental samples with self-absorption correction is described. The method is based on the comparison of two γ peak activities coming from other natural radionuclides, usually present in environmental samples. We have analyzed the dependence of the self-absorption correction factor for the 210Pb activity on the activity ratios of 911 and 209 keV peaks and 609 and 295 keV peaks coming from nuclides of 238U or 232Th rows, present in typical environmental samples.