Volcanic ash has the capacity to impact human health, livestock, crops and infrastructure, including international air traffic. For recent major eruptions, information on the volcanic ash plume has been combined with relatively coarse-resolution meteorological model output to provide simulations of regional ash dispersal, with reasonable success on the scale of hundreds of kilometres. However, to predict and mitigate these impacts locally, significant improvements in modelling capability are required. Here, we present results from a dynamic meteorological-ash-dispersion model configured with sufficient resolution to represent local topographic and convectively-forced flows. We focus on an archetypal volcanic setting, Soufrière, St Vincent, and use the exceptional historical records of the 1902 and 1979 eruptions to challenge our simulations. We find that the evolution and characteristics of ash deposition on St Vincent and nearby islands can be accurately simulated when the wind shear associated with the trade wind inversion and topographically-forced flows are represented. The wind shear plays a primary role and topographic flows a secondary role on ash distribution on local to regional scales. We propose a new explanation for the downwind ash deposition maxima, commonly observed in volcanic eruptions, as resulting from the detailed forcing of mesoscale meteorology on the ash plume.

The number of large urban agglomerations is steadily increasing worldwide. At a local scale, their emissions lead to air pollution, directly affecting people's health. On a global scale, their emissions lead to an increase of greenhouse gases, affecting climate. In this context, in 2017 and 2018, the airborne campaign EMeRGe (Effect of Megacities on the transport and transformation of pollutants on the Regional to Global scales) investigated emissions of European and Asian major population centres (MPCs) to improve the understanding and predictability of pollution outflows. Here, we present two methods to identify and characterise pollution outflows probed during EMeRGe. First, we use a set of volatile organic compounds (VOCs) as chemical tracers to characterise air masses by specific source signals, i.e. benzene from anthropogenic pollution of targeted regions, acetonitrile from biomass burning (BB, primarily during EMeRGe-Asia), and isoprene from fresh biogenic signals (primarily during EMeRGe-Europe. Second, we attribute probed air masses to source regions and estimate their individual contribution by constructing and applying a simple emission uptake scheme for the boundary layer which combines FLEXTRA back trajectories and EDGAR carbon monoxide (CO) emission rates (acronyms are provided in the Appendix). During EMeRGe-Europe, we identified anthropogenic pollution outflows from northern Italy, southern Great Britain, the Belgium–Netherlands–Ruhr (BNR) area and the Iberian Peninsula. Additionally, our uptake scheme indicates significant long-range transport of pollution from the USA and Canada. During EMeRGe-Asia, the pollution outflow is dominated by sources in China and Taiwan, but BB signals from Southeast Asia and India contribute as well. Outflows of pre-selected MPC targets are identified in less than 20 % of the sampling time, due to restrictions in flight planning and constraints of the measurement platform itself. Still, EMeRGe combines in a unique way near- and far-field measurements, which show signatures of local and distant sources, transport and conversion fingerprints, and complex air mass compositions. Our approach provides a valuable classification and characterisation of the EMeRGe dataset, e.g. for BB and anthropogenic influence of potential source regions and paves the way for a more comprehensive analysis and various model studies.

A high-resolution forecast methodology for the ash hazard at Sakurajima volcano, Japan, is presented. The methodology employs a combined modeling approach and utilizes eruption source parameters estimated by geophysical observations from Sakurajima, allowing for a proactive approach in forecasting. The Weather Research and Forecasting (WRF) model is used to downscale Japan Meteorological Agency (JMA) forecast data over the area of interest. The high-resolution meteorological data are then used in FALL3D model to provide a forecast for the ash dispersal and deposition. The methodology is applied for an eruption that occurred on June 16, 2018. Disdrometer observations of ashfall are used along with ash dispersal modeling to inform the choice of the total grain size distribution (TGSD). A series of pseudo-forecast ash dispersal simulations are then carried out using the proposed methodology and estimated TGSD, initialized with meteorological forecast data released up to ∼13 hours before the eruption, with results showing surprising consistency up to ∼10 hours before the eruption. Using forecast data up to 4 hours before the eruption was seen to constrain observation to model ratios within a factor of 2–4 depending on the timing of simulation and location. A number of key future improvements for the methodology are also highlighted.

Volcanic plumes from small and moderate eruptions represent a challenge in the study of plume morphology due to eruption source parameter uncertainties and atmospheric influence. Sakurajima volcano, Japan, features such activity and due to its continuous eruptions in the recent years provides an ideal natural laboratory. A data set of 896 eruptions between 2009 and 2016 with well‐constrained plume heights, estimated erupted mass, and associated atmospheric conditions has been compiled. Plume heights ranged between 1,500 and 5,000 m and mainly developed under stable atmospheric stratification and low background wind speeds. The eruptions presented in the database were used to drive FPLUME, a 1‐D integral volcanic plume model, to study the simulated plume morphology. FPLUME was seen to provide consistent results under stable atmospheric stratification. A method for the real‐time monitoring of erupted mass used in the Sakurajima observatory was seen to provide appropriate first guess estimates for the eruptions, showing agreement with analytical and simulated mass flow rate calculations. Volcanic plumes from Sakurajima show significant influence by the atmospheric environment. The plume scaling parameter (Π) was used to characterize the expected degree of plume bending with results correlating well against modeled plume angles. The vertical wind profile was seen to have a significant impact on the resolved plume. Wind shear characteristics were seen to have a mechanical effect on the plume, aiding or inhibiting bending. Finally, potential issues were identified in simulations under unstable atmospheric conditions as the model either failed to provide a solution or overestimated the plume height.