Near-field microscopy techniques operating in the terahertz (THz) frequency band offer the tantalizing possibility of visualizing with nanometric resolution the localized THz fields supported by individual resonators, micro-structured surfaces, and metamaterials. Such capabilities promise to underpin the future development and characterization of a wide range of devices, including THz emitters, detectors, optoelectronic modulators, sensors, and novel optical components. In this work, we report scattering-type scanning near-field optical microscopy using a THz-frequency quantum cascade laser (QCL) to probe coherently the localized field supported by individual micro-resonator structures. Our technique demonstrates deep sub-wavelength mapping of the field distribution associated with in-plane resonator modes in plasmonic dipole antennas and split ring resonator structures. By exploiting electronic tuning of the QCL in conjunction with the coherent self-mixing effect in these lasers, we are able to resolve both the magnitude and the phase of the out-of-plane field. We, furthermore, show that the elliptically polarized state of the QCL field can be exploited for the simultaneous excitation and measurement of plasmonic resonances in these structures while suppressing the otherwise dominant signal arising from the local material permittivity.
We investigate the effect of substrate etching on terahertz frequency range metamaterials using finite-element method simulations. A blue shift was found in the metamaterial resonance with increasing substrate etch depth, caused by a decrease in the effective refractive index. The relative contribution of the substrate’s refractive index to the effective refractive index was obtained as a function of the etch depth, finding that the decay length of the electric field magnitude below the LC gap is larger for the etched metamaterials due to their lower effective refractive index. We suggest designs for a terahertz metamaterial liquid sensor utilizing substrate etching which shows a significant enhancement in sensitivity compared to unetched sensors using ethanol as an example analyte. The sensitivity of the liquid sensor was enhanced by up to ~6.7-fold, from 76.4 to 514.5 GHz/RIU, for an ethanol liquid layer with a thickness of 60 μm by the incorporation of a substrate etch depth of 30 µm. Since the region of space close to the metamaterial is the most sensitive, however, we find that for small liquid thicknesses, larger etch depths can act to decrease sensitivity, and provide quantitative estimates of this effect.
We propose a novel method for detecting microplastic particles in water using terahertz metamaterials. Fluidic channels are employed to flow the water, containing polystyrene spheres, on the surface of the metamaterials. Polystyrene spheres are captured only near the gap structure of the metamaterials as the gap areas are functionalized. The resonant frequency of terahertz metamaterials increased while we circulated the microplastic solution, as polystyrene spheres in the solution are attached to the metamaterial gap areas, which saturates at a specific frequency as the gap areas are filled by the polystyrene spheres. Experimental results were revisited and supported by finite-difference time-domain simulations. We investigated how this method can be used for the detection of microplastics with various solution densities. The saturation time of the resonant frequency shift was found to decrease, while the saturated resonant frequency shift increased as the solution density increased.
We investigate the use of finite-element simulations as a novel method for determining the dielectric property of target materials in the terahertz (THz) frequency range using split-ring resonator (SRR) sensing elements integrated into a planar Goubau line (PGL) waveguide. Five such SRRs were designed to support resonances at specific target frequencies. The origin of resonance modes was identified by investigating the electric field distribution and surface current modes in each SRR. Red-shifts were found in the resonances upon deposition of overlaid test dielectric layers that saturated for thicknesses above 10 µm. We also confirmed that the SRRs can work as independent sensors by depositing the analyte onto each individually. The relation between the permittivity of the target material and the saturated resonant frequency was obtained in each case, and was used to extract the permittivity of a test dielectric layer at six different frequencies in the range of 200–700 GHz as an example application. Our approach enables the permittivity of small volumes of analytes to be determined at a series of discrete frequencies up to ~1 THz.
31 March 2023 in IEEE Transactions on Terahertz Science and Technology
The potential of terahertz (THz) spectroscopy and imaging in skin cancer detection and mainly basal cell carcinoma (BCC), the most common type of skin cancer, was previously studied. Thanks to the significant absorption of THz waves by hydrogen bonds of water and the higher hydration of tumors than normal skin, it is considered an ideal non-invasive tool for early cancer detection. Despite this potential, there is a lack of study on the THz characterization of treated tumors with anticancer drugs to constitute innovative approaches for chemotherapeutic research, and this is an inspiration for the current study. Previous THz spectroscopy measurements are based on freshly excised tissue and suffer from environmental impacts on tissue and also limit performing a thorough analysis of the effect of different biological parameters. Thus, we have cultured a three-dimensional (3D) organotypic model of BCC tumor to study the THz electromagnetic parameters of tumor in different stages along with the impact of AG1478 anticancer drug on its THz spectra. Measurements are performed in the frequency range of 0.4 to 1.6 THz, and the corresponding refractive index, absorption coefficient, and complex permittivity of normal skin, BCC, and treated BCC have been compared. Furthermore, an enhanced combinational optimization algorithm is developed to calculate the parameters of the double Debye (DD) dielectric model to explain better the discrimination of treated and untreated tumors with normal skin.
We have used finite-element methods to design and simulate a tunable terahertz frequency range band-stop filter based on coupled split-ring resonators integrated into planar Goubau-line waveguide. Two split-ring resonators with different geometrical lengths and gap widths were designed to resonate at the same frequency. When the two resonators were coupled, resonance splitting was observed in the transmission spectra controlled by the distance between them. The electric field distribution and surface current modes in the coupled resonators were used to identify the origin of the resonance modes. In order to dynamically tune the coupled resonance frequencies, a cantilevered microelectromechanical scheme is proposed, in which the radius of curvature of one split-ring resonator is adjusted with respect to a fixed second split-ring resonator. The coupling strength of the coupled resonators was investigated as a function of the relative separation of the resonators revealing a dispersion relation that shows anti-crossing of the coupled resonances as the cantilever bends.