Ghost imaging, based on single-pixel detection and multiple pattern illumination, is a crucial investigative tool in difficult-to-access wavelength regions. In the terahertz domain, where high-resolution imagers are mostly unavailable, ghost imaging is an optimal approach to embed the temporal dimension, creating a “hyperspectral” imager. In this framework, high resolution is mostly out of reach. Hence, it is particularly critical to developing practical approaches for microscopy. Here we experimentally demonstrate time-resolved nonlinear ghost imaging, a technique based on near-field, optical-to-terahertz nonlinear conversion and detection of illumination patterns. We show how space–time coupling affects near-field time-domain imaging, and we develop a complete methodology that overcomes fundamental systematic reconstruction issues. Our theoretical-experimental platform enables high-fidelity subwavelength imaging and carries relaxed constraints on the nonlinear generation crystal thickness. Our work establishes a rigorous framework to reconstruct hyperspectral images of complex samples inaccessible through standard fixed-time methods.

Laser cavity-soliton microcombs are robust optical pulsed sources, usually implemented with a microresonator-filtered fibre laser. In such a configuration, a nonlinear microcavity converts the narrowband pulse resulting from bandwidth-limited amplification to a background-free broadband microcomb. Here, we theoretically and experimentally study the soliton conversion efficiency between the narrowband input pulse and the two outputs of a four-port integrated microcavity, namely the ‘Drop’ and ‘Through’ ports. We simultaneously measure on-chip, single-soliton conversion efficiencies of 45% and 25% for the two broadband comb outputs at the ‘Drop’ and ‘Through’ ports of a 48.9 GHz free-spectral range micro-ring resonator, obtaining a total conversion efficiency of 72%.

Laser cavity-solitons can appear in systems comprised of a nonlinear microcavity nested within an amplifying fiber loop. These states are robust and self-emergent and constitute an attractive class of solitons that are highly suitable for microcomb generation. Here, we present a detailed study of the free-running stability properties of the carrier frequency and repetition rate of single solitons, which are the most suitable states for developing robust ultrafast and high repetition rate comb sources. We achieve free-running fractional stability on both optical carrier and repetition rate (i.e., 48.9 GHz) frequencies on the order of $10^{-9}$ for a 1 s gate time. The repetition rate results compare well with the performance of state-of-the-art (externally driven) microcomb sources, and the carrier frequency stability is in the range of performance typical of modern free-running fiber lasers. Finally, we show that these quantities can be controlled by modulating the laser pump current and the cavity length, providing a path for active locking and long-term stabilization.

Terahertz (THz) imaging is a rapidly emerging field, thanks to many potential applications in diagnostics, manufacturing, medicine and material characterisation. However, the relatively coarse resolution stemming from the large wavelength limits the deployment of THz imaging in micro- and nano-technologies, keeping its potential benefits out-of-reach in many practical scenarios and devices. In this context, single-pixel techniques are a promising alternative to imaging arrays, in particular when targeting subwavelength resolutions. In this work, we discuss the key advantages and practical challenges in the implementation of time-resolved nonlinear ghost imaging (TIMING), an imaging technique combining nonlinear THz generation with time-resolved time-domain spectroscopy detection. We numerically demonstrate the high-resolution reconstruction of semi-transparent samples, and we show how the Walsh–Hadamard reconstruction scheme can be optimised to significantly reduce the reconstruction time. We also discuss how, in sharp contrast with traditional intensity-based ghost imaging, the field detection at the heart of TIMING enables high-fidelity image reconstruction via low numerical-aperture detection. Even more striking—and to the best of our knowledge, an issue never tackled before—the general concept of “resolution” of the imaging system as the “smallest feature discernible” appears to be not well suited to describing the fidelity limits of nonlinear ghost-imaging systems. Our results suggest that the drop in reconstruction accuracy stemming from non-ideal detection conditions is complex and not driven by the attenuation of high-frequency spatial components (i.e., blurring) as in standard imaging. On the technological side, we further show how achieving efficient optical-to-terahertz conversion in extremely short propagation lengths is crucial regarding imaging performance, and we propose low-bandgap semiconductors as a practical framework to obtain THz emission from quasi-2D structures, i.e., structure in which the interaction occurs on a deeply subwavelength scale. Our results establish a comprehensive theoretical and experimental framework for the development of a new generation of terahertz hyperspectral imaging devices.

The interest in surface terahertz emitters lies in their extremely thin active region, typically hundreds of atomic layers, and the agile surface scalability. The ultimate limit in the achievable emission is determined by the saturation of the several different mechanisms concurring to the THz frequency conversion. Although there is a very prolific debate about the contribution of each process, surface optical rectification has been highlighted as the dominant process at high excitation, but the effective limits in the conversion are largely unknown. The current state of the art suggests that in field-induced optical rectification a maximum limit of the emission may exist and it is ruled by the photocarrier induced neutralisation of the medium's surface field. This would represent the most important impediment to the application of surface optical rectification in high-energy THz emitters. We experimentally unveil novel physical insights in the THz conversion at high excitation energies mediated by the ultrafast surface optical rectification process. The main finding is that the expected total saturation of the Terahertz emission vs pump energy does not actually occur. At high energy, the surface field region contracts towards the surface. We argue that this mechanism weakens the main saturation process, re-establishing a clearly observable quadratic dependence between the emitted THz energy and the excitation. This is relevant in enabling access to intense generation at high fluences.

We study the interaction of a laser cavity-soliton microcomb with an externally coupled, co-propagating tunable CW pump, observing parametric Kerr interactions which lead to the formation of both a cross-phase modulation and a four-wave mixing replica of the laser cavity-soliton. We compare and explain the dependence of the microcomb spectra from both the cavity-soliton and pump parameters, demonstrating the ability to adjust the microcomb externally without breaking or interfering with the soliton state. The parametric nature of the process agrees with numerical simulations. The parametric extended state maintains the typical robustness of laser-cavity solitons.