In femtosecond pump-probe measurements, the appearance of coherent phonon oscillations at 4.5 and 6.0 THz indicating the rutile metal phase of does not occur simultaneously with the first-order metal-insulator transition (MIT) near . The monoclinic and correlated metal (MCM) phase between the MIT and the structural phase transition (SPT) is generated by a photoassisted hole excitation, which is evidence of the Mott transition. The SPT between the MCM phase and the rutile metal phase occurs due to subsequent Joule heating. The MCM phase can be regarded as an intermediate nonequilibrium state.
We report spatial domain measurements of the damping of surface-plasmon excitations in metal films with periodic nanohole arrays. The measurements reveal a short coherent propagation length of a few inside nanohole arrays, consistent with delays of about 10 fs in ultrafast transmission experiments. This implies that the transmission spectra of the entire plasmonic band-gap structure are homogeneously broadened by radiative damping of surface-plasmon excitations. We show that a Rayleigh-like scattering of surface plasmons by the periodic hole array is the microscopic origin of this damping, allowing the reradiation rate to be controlled.
We have investigated experimentally the effects of n-type impurities such as Al and H on the magnetic properties of ZnCoO. The carrier density changes slightly upon the introduction of hydrogen but increases significantly in the case of Al. A measurement of magnetic circular dichroism indicates that, of the two impurities, only H induces ferromagnetism in ZnCoO. Our experimental data suggest that, unlike Al, H plays an important role in the enhancement of ferromagnetic spin-spin interactions that goes much beyond a carrier-mediated effect.