An effective semianalytical method for analyzing the Cartesian multipole contributions in light transmission and reflection spectra of flat metasurfaces composed of identical nanoparticles is developed and demonstrated. The method combines numerical calculation of metasurface reflection and transmission coefficients with their multipole decompositions. The developed method is applied for the multipole analysis of reflection and transmission spectra of metasurfaces composed of silicon nanocubes or nanocones. In the case of nanocubes, we numerically demonstrate a “lattice invisibility effect,” when light goes through the metasurface almost without amplitude and phase perturbations with the simultaneous excitation of nanoparticles' multipole moments. The effect is realized due to destructive interference between the fields generated by the basic multipole moments of nanoparticles in the backward and forward directions. For metasurfaces composed of conical nanoparticles, we show that their transmission coefficient does not depend on illumination direction. In contrast, the reflection and absorption can be different for the illumination from different metasurface sides, which is associated with the excitation of different multipoles. We believe our results could be useful for analysis and understanding of the electromagnetic properties of nanoparticle arrays and pave the way for the design of novel metasurfaces for various optical applications.
All-dielectric resonant nanophotonics lies at the heart of modern optics and nanotechnology due to the unique possibilities to control scattering of light from high-index dielectric nanoparticles and metasurfaces. One of the important concepts of dielectric Mie-resonant nanophotonics is associated with the Kerker effect that drives the unidirectional scattering of light from nanoantennas and Huygens metasurfaces. Here we suggest and demonstrate experimentally a novel effect manifested in the nearly complete simultaneous suppression of both forward and backward scattered fields. This effect is governed by the Fano resonance of an electric dipole and off-resonant quadrupoles, providing necessary phases and amplitudes of the scattered fields to achieve the transverse scattering. We extend this concept to dielectric metasurfaces that demonstrate zero reflection with transverse scattering and strong field enhancement for resonant light filtering, nonlinear effects, and sensing.
On‐chip nanophotonic devices are a class of devices capable of controlling light on a chip to realize performance advantages over ordinary building blocks of integrated photonics. These ultra‐fast and low‐power nanoscale optoelectronic devices are aimed at high‐performance computing, chemical, and biological sensing technologies, energy‐efficient lighting, environmental monitoring and more. They are increasingly becoming an attractive building block in a variety of systems, which is attributed to their unique features of large evanescent field, compactness, and most importantly their ability to be configured according to the required application. This review summarizes recent advances of integrated nanophotonic devices and their demonstrated applications, including but not limited to, mid‐infrared and overtone spectroscopy, all‐optical processing on a chip, logic gates on a chip, and cryptography on a chip. The reviewed devices open up a new chapter in on‐chip nanophotonics and enable the application of optical waveguides in a variety of optical systems, thus are aimed at accelerating the transition of nanophotonics from academia to the industry.
Spectral multipole resonances of parallelepiped-, pyramid-, and cone-like shaped silicon nanoparticles excited by linearly polarized light waves are theoretically investigated. The numerical finite element method is applied for the calculations of the scattering cross sections as a function of the nanoparticles geometrical parameters. The roles of multipole moments (up to the third order) in the scattering process are analyzed using the semianalytical multipole decomposition approach. The possibility of scattering pattern configuration due to the tuning of the multipole contributions to the total scattered waves is discussed and demonstrated. It is shown that cubic nanoparticles can provide a strong isotropic side scattering with minimization of the scattering in forward and backward directions. In the case of the pyramidal and conical nanoparticles the total suppression of the side scattering can be obtained. It was found that due to the shape factor of the pyramidal and conical nanoparticles their electric toroidal dipole resonance can be excited in the spectral region of the first electric and magnetic dipole resonances. The influence of the incident light directions on the optical response of the pyramidal and conical nanoparticles is discussed. The obtained results provide important information that can be used for the development of nanoantennas with improved functionality due to the directional scattering effects.
We have discovered a strong increase in the intensity of the chemiluminescence of a luminol flow and a dramatic modification of its spectral shape in the presence of metallic nanoparticles. We observed that pumping gold and silver nanoparticles into a microfluidic device fabricated in polydimethylsiloxane prolongs the glow time of luminol. We have demonstrated that the intensity of chemiluminescence in the presence of nanospheres depends on the position along the microfluidic serpentine channel. We show that the enhancement factors can be controlled by the nanoparticle size and material. Spectrally, the emission peak of luminol overlaps with the absorption band of the nanospheres, which maximizes the effect of confined plasmons on the optical density of states in the vicinity of the luminol emission peak. These observations, interpreted in terms of the Purcell effect mediated by nano-plasmons, form an essential step toward the development of microfluidic chips with gain media. Practical implementation of the discovered effect will include improving the detection limits of chemiluminescence for forensic science, research in biology and chemistry, and a number of commercial applications.
In this Letter, we demonstrate and investigate the Kerker-type effect in high-index dielectric nanoparticles for which the third-order multipoles give a considerable contribution to the light scattering process. It is shown that the Kerker-type effect (strong suppression of the backward light scattering and, simultaneously, resonant forward light scattering) can be associated with the resonant excitation of a toroidal dipole moment in the system. This effect is realized due to the interference of the scattered waves generated by electric, magnetic, and toroidal dipole moments of high-index nanoparticles.