Flexible sensors with low fabrication cost, high sensitivity, and good stability are essential for the development of smart devices for wearable electronics, soft robotics, and electronic skins. Herein, we report a nanocomposite material based on carbon nanotube and metal oxide semiconductor for ultraviolet (UV) sensing applications, and its sensing behavior. The sensors were prepared by a screen-printing process under a low-temperature curing condition. The formation of a conducting string node and a sensing node could enhance a UV sensing response, which could be attributed to the uniform mixing of functionalized multi-walled carbon nanotubes and zinc oxide nanoparticles. A fabricated device has shown a fast response time of 1.2 s and a high recovery time of 0.8 s with good mechanical stability.