Energy, pulse duration, and frequency of the spectral maximum are important characteristics of pulsed terahertz radiation. The unipolarity of radiation is another characteristic that is paid less attention to. This paper demonstrates possible ways how to determine the presence of unipolarity in the radiation of pulsed terahertz sources. The first approach is based on integrating the time dependence of the field strength in the far zone obtained experimentally. The second approach uses radio-technical equipment by means of recording low-frequency components of pulses, which exist in the unipolar terahertz radiation. The results of experiments are presented with recording the unipolar component of THz pulses by both methods. The existence of unipolarity is shown for pulses from some types of terahertz radiation sources. Estimations are made for the electric area and the degree of unipolarity of the pulsed radiation for the first time.

Speckle patterns can be very promising for many applications due to their unique properties. This paper presents the possibility of numerically and experimentally formation of speckle patterns using broadband THz radiation. Strong dependence of the statistical parameters of speckles, such as size and sharpness on the parameters of the diffuser are demonstrated: the correlation length and the mean square deviation of the phase surface inhomogeneity. As the surface correlation length is increasing, the speckle size also increases and its sharpness goes down. Alternatively, the magnification of the standard deviation of the surface height leads to the speckle size diminishing and growth of the speckle sharpness. The dimensions of the experimentally formed speckles correspond to the results of numerical simulation. The possibility of utilizing formed speckle patterns for the implementation of the ghost imaging technique has been demonstrated by methods of numerical modeling.

A method is proposed for accelerating measurements for ghost imaging reconstruction of objects using spectral multiplexing of speckle patterns formed by broadband terahertz (THz) radiation. The presented method aims at the challenge of a sufficiently large number of measurements, and increases the correlation between reference and reconstructed images. It is experimentally shown that unique speckle patterns for individual frequencies can be formed by broadband THz radiation while propagating through a random phase plate. It is shown by numerical simulation that these speckle patterns can be used to decrease the number of diffusers required by more than one order compared to the integrated method. The possibility of using electro-optical detection in the proposed technique reduces the number of measurements. For example, for the spectral range from 0.2 to 1.2 THz, there is a more than 20-fold decrease in the number of diffusers used.

Metal halide perovskite nanocrystals (NCs) attract much attention for light-emitting applications due to their exceptional optical properties. More recently, perovskite NCs have begun to be considered a promising material for nonlinear optical applications. Numerous strategies have recently been developed to improve the properties of metal halide perovskite NCs. Among them, B-site doping is one of the most promising ways to enhance their brightness and stability. However, there is a lack of study of the influence of B-site doping on the nonlinear optical properties of inorganic perovskite NCs. Here, we demonstrate that Cd²⁺ doping simultaneously improves both the linear (higher photoluminescence quantum yield, larger exciton binding energy, reduced trap states density, and faster radiative recombination) and nonlinear (higher two- and three-photon absorption cross-sections) optical properties of CsPbBr₃ NCs. Cd²⁺ doping results in a two-photon absorption cross-section, reaching 2.6 × 10⁶ Goeppert-Mayer (GM), which is among the highest reported for CsPbBr₃ NCs.

Due to their high resonant third-order nonlinear response, lead sulfide quantum dots (QDs) are potential materials for applications in the field of nonlinear optics. In this paper, we implement the Z-scan method to study the resonant nonlinear response of lead sulfide QDs in colloidal solutions. We managed to measure the purely intrinsic resonant nonlinear response, free of thermal contribution. We report that the lead sulfide QD third-order nonlinear response per QD shows an unconventional increase. A figure of merit for QD nonlinearity grows as a power function with a factor of 2.9.

Lead halide perovskite nanoplatelets (NPls) attract significant attention due to their exceptional and tunable optical properties. Doping is a versatile strategy for modifying and improving the optical properties of colloidal nanostructures. However, the protocols for B-site doping have been rarely reported for 2D perovskite NPls. In this work, we investigated the post-synthetic treatment of CsPbBr₃ NPls with different Cd²⁺ sources. We show that the interplay between Cd²⁺ precursor, NPl concentrations, and ligands determines the kinetics of the doping process. Optimization of the treatment allows for the boosting of linear and nonlinear optical properties of CsPbBr₃ NPls via doping or/and surface passivation. At a moderate doping level, both the photoluminescence quantum yield and two-photon absorption cross section increase dramatically. The developed protocols of post-synthetic treatment with Cd²⁺ facilitate further utilization of perovskite NPls in nonlinear optics, photonics, and lightning.