We have calculated a complete set of primary fission fragment mass yields, $Y\left(A\right)$, for heavy nuclei across the chart of nuclides, including those of particular relevance to the rapid neutron capture process ($r$ process) of nucleosynthesis. We assume that the nuclear shape dynamics are strongly damped, which allows for a description of the fission process via Brownian shape motion across nuclear potential-energy surfaces. The macroscopic energy of the potential was obtained with the Finite-Range Liquid-Drop Model (FRLDM), while the microscopic terms were extracted from the single-particle level spectra in the fissioning system by the Strutinsky procedure for the shell energies and the BCS treatment for the pairing energies. For each nucleus considered, the fission fragment mass yield, $Y\left(A\right)$, is obtained from 50 000 to 500 000 random walks on the appropriate potential-energy surface. The full mass and charge yield, $Y(Z,A)$, is then calculated by invoking the Wahl systematics. With this method, we have calculated a comprehensive set of fission-fragment yields from over 3800 nuclides bounded by $80\le Z\le 130$ and $A\le 330$; these yields are provided as an ASCII formatted database in the Supplemental Material. We compare our yields to known data and discuss general trends that emerge in low-energy fission yields across the chart of nuclides.

During nuclear fission, a heavy nucleus splits into two rotating fragments. The associated angular momentum is large, yet the mechanism of its generation and its dependence on the mass of fragments remain poorly understood. In this Letter, we provide the first microscopic calculations of angular-momentum distributions in fission fragments for a wide range of fragment masses. For the benchmark case of ${}^{239}\mathrm{Pu}(n_{\text{th}},f)$, we find that the angular momentum of the fragments is largely determined by the nuclear shell structure and deformation, and that the heavy fragments therefore typically carry less angular momentum than their light partners. We use the fission model freya to simulate the emission of neutrons and photons from the fragments. The dependence of the angular momenta on fragment mass after the emission of neutrons and statistical photons is linear for the heavy fragments and either constant or weakly linear for the light fragments, consistent with the universal sawtooth pattern suggested by recent experimental data. Finally, we observe that using microscopic angular-momentum distributions modifies the number of emitted photons significantly.

Background: The role of angular momentum in fission has long been discussed but the observable effects are difficult to quantify.

We recently introduced a fluid-dynamical model for simulating relativistic nuclear collisions in the presence of a first-order phase transition and made explorative studies of head-on lead-lead collisions. We give here a more detailed account of this novel theoretical tool and carry out more exhaustive studies of the phase-separation dynamics. Extracting the density enhancement caused by the spinodal instabilities, the associated clump size distribution, and the resulting transverse flow velocity, we examine the sensitivity of these quantities to the strength of the gradient term that promotes the phase separation, to the details of the initial density fluctuations that form the seeds for the subsequent amplification, and to the equation of state.

We discuss how the measurement of photon angular correlations can reveal information about the orientation of the fission fragment angular momenta. Photons from identified stretched $E2$ collective transitions in even-even fission product nuclei are particularly suitable because they do not affect the orientation of the nuclear spin. Their angular distribution relative to the direction of a fission fragment may reveal the orientation of the fragment spins relative to the fission axis. A novel means of probing the correlated fission fragment spins is the distribution of the opening angle between $E2$ photons from even-even partner fragments which reveals the mutual correlation of the fragment spins, if the photon helicities can be determined, demonstrating the potential power of helicity measurements in fission.