With the proposal of dual-wavelength pumping (DWP) scheme, DWP Er:ZBLAN fiber lasers at 3.5 μm have become a fascinating area of research. However, limited by the absence of suitable saturable absorber, passively Q-switched and mode-locked fiber lasers have not been realized in this spectral region. Based on the layer-dependent bandgap and excellent photoelectric characteristics of black phosphorus (BP), BP is a promising candidate for saturable absorber near 3.5 μm. Here, we fabricated a 3.5-μm saturable absorber mirror (SAM) by transferring BP flakes onto a Au-coated mirror. With the as-prepared BP SAM, we realized Q-switching and mode-locking operations in the DWP Er:ZBLAN fiber lasers at 3.5 μm. To the best of our knowledge, it is the first time to achieve passively Q-switched and mode-locked pulses in 3.5 μm spectral region. The research results will not only promote the development of 3.5-μm pulsed fiber lasers but also open the photonics application of two-dimensional materials in this spectral region.

We demonstrate a noncollinear optical parametric chirped-pulse amplification scheme for generating high-peak-power tunable mid-infrared (IR) pulses. The high-gain ${\mathrm{LiNbO}}_3$-based noncollinear parametric amplifier, seeded by a tunable femtosecond optical parametric amplifier, provides a wide wavelength tuning range from 3.3 to 3.95 μm and a large saturated gain of over 4000 in a single-stage amplifier. The compressed mid-IR pulse has a pulse energy of 13.3 mJ and pulse duration of 111 fs, with a peak power as high as 120 GW. To the best of our knowledge, this is the highest peak power ever reported for 3–5 μm tunable mid-IR lasers.

In past years, rare-earth-doped fluoride fiber lasers (FFLs) have developed rapidly in the mid-infrared (mid-IR) region. However, due to the lack of fiber optic devices and challenge of fluoride fiber splicing, most mid-IR FFLs have been demonstrated with free-space optic elements, limiting the advantages of all-fiber lasers for flexible delivery, stability, and compactness. Here, we report, to the best of our knowledge, the first pulsed all-fiber FFL in the mid-IR region. By taking advantage of the integration of black phosphorus flake, stable $Q$-switched and mode-locked pulses were obtained at 2.8 μm wavelength. We believe that this all-fiber design will promote the application of pulsed FFL in the mid-IR region.

Semiconductor saturable absorber mirrors (SESAMs) have been regarded as a revolutionary technology for ultrafast mode-locked lasers, producing numerous landmark laser breakthroughs. However, the operating wavelength of existing SESAMs is limited to less than 3 µm. In this study, we create a 3–5 µm mid-infrared (MIR) SESAM by engineering an InAs/GaSb type-II superlattice. Bandgap engineering and the strong coupling between potential wells in a superlattice enable a broadband response of saturable absorption in the 3–5 µm spectral range. Using the fabricated SESAM, we realize a SESAM mode-locked Er:ZBLAN fiber laser at 3.5 µm, which delivers MIR ultrashort pulses with high long-term stability. The breakthrough of SESAM fabrication in the MIR will promote the development of MIR ultrafast coherent sources and related application fields.

Quasi-parametric chirped pulse amplification (QPCPA) is a new scheme that enables the amplification of chirped signal pulses without back conversion by depleting the idler pulses. In this paper, we present a numerical study on the bandwidth, efficiency, and robustness of QPCPA. Self-locked phase among the interacting waves is found to be the underlying mechanism for the suppression of back conversion, which allows signal efficiency approaching to the quantum limit even under the phase-mismatch condition, and thus greatly increases the phase-mismatch tolerance of QPCPA. We demonstrate that QPCPA can break through the trade-off between the efficiency and bandwidth encountered in conventional optical parametric amplification, hence supporting highly efficient amplification of few-cycle pulses.

Real-time pulse-contrast observation with a high dynamic range is a prerequisite to tackle the contrast challenge in ultra-high peak-power lasers. However, the commonly used delay-scanning cross-correlator (DSCC) can only provide the time-consumed measurements for repetitive lasers. Single-shot cross-correlator (SSCC) becomes essential in optimizing laser systems and exploring contrast mechanisms. Here we report our progress in developing SSCC towards its practical use. By integrating both the techniques of scattering-noise reduction and sensitive parallel detection into SSCC, we demonstrate a high dynamic range of >10¹⁰, which, to our best knowledge, is the first demonstration of an SSCC with a dynamic range comparable to that of commercial DSCCs. The comparison of high-dynamic measurement performances between SSCC and a standard DSCC (Sequoia, Amplitude Technologies) is also carried out on a 200 TW Ti:sapphire laser, and the consistency of results verifies the veracity of our SSCC.