Downward surface solar radiation (SSR) trends for the first decade of the 2000s were computed using a radiative transfer model and satellite and reanalysis input data and were validated against measurements from the reference global station networks Global Energy Balance Archive (GEBA) and Baseline Surface Radiation Network (BSRN). Under all-sky conditions, in spite of a somewhat patchy structure of global dimming and brightening (GDB), an overall dimming was found that is weaker in the Northern than in the Southern Hemisphere (−2.2 and −3.1 W m⁻², respectively, over the 2001–2009 period). Dimming is observed over both land and ocean in the two hemispheres, but it is more remarkable over land areas of the Southern Hemisphere. The post-2000 dimming is found to have been primarily caused by clouds, and secondarily by aerosols, with total cloud cover contributing −1.4 W m⁻² and aerosol optical thickness −0.7 W m⁻² to the global average dimming of −2.65 W m⁻². The evaluation of the model-computed GDB against BSRN and GEBA measurements indicates a good agreement, with the same trends for 65% and 64% of the examined stations, respectively. The obtained model results are in line with other studies for specific world regions and confirm the occurrence of an overall solar dimming over the globe during the first decade of 21st century. This post-2000 dimming has succeeded the global brightening observed in the 1990s and points to possible impacts on the ongoing global warming and climate change.

A satellite-based algorithm is developed and used to determine the presence of dust aerosols on a global scale. The algorithm uses as input aerosol optical properties from the MOderate Resolution Imaging Spectroradiometer (MODIS)-Aqua Collection 6.1 and Ozone Monitoring Instrument (OMI)-Aura version v003 (OMAER-UV) datasets and identifies the existence of dust aerosols in the atmosphere by applying specific thresholds, which ensure the coarse size and the absorptivity of dust aerosols, on the input optical properties. The utilized aerosol optical properties are the multiwavelength aerosol optical depth (AOD), the Aerosol Absorption Index (AI) and the Ångström Exponent (a). The algorithm operates on a daily basis and at 1° × 1° latitude-longitude spatial resolution for the period 2005–2019 and computes the absolute and relative frequency of the occurrence of dust. The monthly and annual mean frequencies are calculated on a pixel level for each year of the study period, enabling the study of the seasonal as well as the inter-annual variation of dust aerosols’ occurrence all over the globe. Temporal averaging is also applied to the annual values in order to estimate the 15-year climatological mean values. Apart from temporal, a spatial averaging is also applied for the entire globe as well as for specific regions of interest, namely great global deserts and areas of desert dust export. According to the algorithm results, the highest frequencies of dust occurrence (up to 160 days/year) are primarily observed over the western part of North Africa (Sahara), and over the broader area of Bodélé, and secondarily over the Asian Taklamakan desert (140 days/year). For most of the study regions, the maximum frequencies appear in boreal spring and/or summer and the minimum ones in winter or autumn. A clear seasonality of global dust is revealed, with the lowest frequencies in November–December and the highest ones in June. Finally, an increasing trend of global dust frequency of occurrence from 2005 to 2019, equal to 56.2%, is also found. Such an increasing trend is observed over all study regions except for North Middle East, where a slight decreasing trend (−2.4%) is found.

Vertical profiling of aerosol particles was performed during the PANhellenic infrastructure for Atmospheric Composition and climatE chAnge (PANACEA) winter campaign (10 January 2020–7 February 2020) over the city of Ioannina, Greece (39.65° N, 20.85° E, 500 m a.s.l.). The middle-sized city of Ioannina suffers from wintertime air pollution episodes due to biomass burning (BB) domestic heating activities. The lidar technique was applied during the PANACEA winter campaign on Ioannina city, to fill the gap of knowledge of the spatio-temporal evolution of the vertical mixing of the particles occurring during these winter-time air pollution episodes. During this campaign the mobile single-wavelength (532 nm) depolarization Aerosol lIdAr System (AIAS) was used to measure the spatio-temporal evolution of the aerosols’ vertical profiles within the Planetary Boundary Layer (PBL) and the lower free troposphere (LFT; up to 4 km height a.s.l.). AIAS performed almost continuous lidar measurements from morning to late evening hours (typically from 07:00 to 19:00 UTC), under cloud-free conditions, to provide the vertical profiles of the aerosol backscatter coefficient (b_aer) and the particle linear depolarization ratio (PLDR), both at 532 nm. In this study we emphasized on the vertical profiling of very fresh (~hours) biomass burning (BB) particles originating from local domestic heating activities in the area. In total, 33 out of 34 aerosol layers in the lower free troposphere were characterized as fresh biomass burning ones of local origin, showing a mean particle linear depolarization value of 0.04 ± 0.02 with a range of 0.01 to 0.09 (532 nm) in a height region 1.21–2.23 km a.s.l. To corroborate our findings, we used in situ data, particulate matter (PM) concentrations (PM_2.5) from a particulate sensor located close to our station, and the total black carbon (BC) concentrations along with the respective contribution of the fossil fuel (BC_ff) and biomass/wood burning (BC_wb) from the Aethalometer. The PM_2.5 mass concentrations ranged from 5.6 to 175.7 μg/m³, while the wood burning emissions from residential heating were increasing during the evening hours, with decreasing temperatures. The BC_wb concentrations ranged from 0.5 to 17.5 μg/m³, with an extremely high mean contribution of BC_wb equal to 85.4%, which in some cases during night-time reached up to 100% during the studied period.

A satellite algorithm able to identify Dust Aerosols (DA) is applied for a climatological investigation of Dust Aerosol Episodes (DAEs) over the greater Mediterranean Basin (MB), one of the most climatologically sensitive regions of the globe. The algorithm first distinguishes DA among other aerosol types (such as Sea Salt and Biomass Burning) by applying threshold values on key aerosol optical properties describing their loading, size and absorptivity, namely Aerosol Optical Depth (AOD), Aerosol Index (AI) and Ångström Exponent (α). The algorithm operates on a daily and 1° × 1° geographical cell basis over the 15-year period 2005–2019. Daily gridded spectral AOD data are taken from Moderate Resolution Imaging Spectroradiometer (MODIS) Aqua Collection 6.1, and are used to calculate the α data, which are then introduced into the algorithm, while AI data are obtained by the Ozone Monitoring Instrument (OMI) -Aura- Near-UV aerosol product OMAERUV dataset. The algorithm determines the occurrence of Dust Aerosol Episode Days (DAEDs), whenever high loads of DA (higher than their climatological mean value plus two/four standard deviations for strong/extreme DAEDs) exist over extended areas (more than 30 pixels or 300,000 km²). The identified DAEDs are finally grouped into Dust Aerosol Episode Cases (DAECs), consisting of at least one DAED. According to the algorithm results, 166 (116 strong and 50 extreme) DAEDs occurred over the MB during the study period. DAEDs are observed mostly in spring (47%) and summer (38%), with strong DAEDs occurring primarily in spring and summer and extreme ones in spring. Decreasing, but not statistically significant, trends of the frequency, spatial extent and intensity of DAECs are revealed. Moreover, a total number of 98 DAECs was found, primarily in spring (46 DAECs) and secondarily in summer (36 DAECs). The seasonal distribution of the frequency of DAECs varies geographically, being highest in early spring over the eastern Mediterranean, in late spring over the central Mediterranean and in summer over the western MB.

In the present study, we used the FORTH deterministic spectral Radiation Transfer Model (RTM) to estimate detailed three-dimensional distributions of the Direct Radiative Effects (DREs) and their consequent modification of the thermal structure of the regional atmosphere during an intense dust episode that took place from 16 to 18 June 2016 over the Mediterranean Basin (MB). The RTM operated on a 3-hourly temporal and 0.5 × 0.625° spatial resolution, using 3-D aerosol optical properties (i.e., aerosol optical depth, single scattering albedo, and asymmetry parameter) and other surface and atmospheric properties from the MERRA-2 reanalysis and cloud properties (i.e., cloud amount, cloud optical depth, and cloud top height) from the ISCCP-H dataset. The model ran with and without dust aerosols, yielding the upwelling and downwelling solar fluxes at the top of the atmosphere, in the atmosphere, and at the Earth’s surface as well as at 50 levels in the atmosphere. The dust direct radiative effect (DDRE) was estimated as the difference between the two (one taking into account all aerosol types and one taking into account all except for dust aerosols) flux outputs. The atmospheric heating rates and subsequent convection induced by dust radiative absorption were calculated at 50 levels to determine how the DDRE affects the thermal structure and dynamics of the atmosphere. The results showed that such a great and intense dust transport event significantly reduces the net surface solar radiation over the MB (by up to 62 W/m² on a daily mean basis, and up to 200 W/m² on an hourly basis, at 12:00 UTC) while increasing the atmospheric solar absorption (by up to 72 W/m² daily and 187 W/m² hourly, at 12:00 UTC). At the top of the atmosphere, both heating (over desert areas) and cooling (over oceanic and other continental areas) are observed due to the significantly different surface albedos. Transported dust causes considerable heating of the region’s atmosphere, which becomes maximum at altitudes where the dust loadings are highest (0.14 K/3 h on 17 June 2016, 12:00 UTC, at 3–5 km above sea level). The dust solar absorption and heating induce a buoyancy as strong as 0.014 m/s², resulting in considerable changes in vertical air motions and possibly contributing to the formation of middle- and high-level clouds over the Mediterranean Basin.

A spatiotemporally extended dust aerosol episode that occurred over the Mediterranean Basin (MB) from 16 to 18 June 2016 is investigated using observational satellite and reanalysis data, focusing on the effects of high dust loads on cloud formation and temperature fields, including the creation of temperature inversions. The atmospheric conditions before and during the 3-day dust aerosol episode case (DAEC) are also analyzed. The dust episode, which is identified using a contemporary satellite algorithm, consists of long-range transport of African dust to the western and central MB. The day to day, before and during the DAEC, atmospheric circulation, dust-cloud interactions, and dust effect on temperature are examined using a variety of Moderate Resolution Imaging Spectroradiometer (MODIS) Level-3 Collection 6.1 satellite and Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) reanalysis data. According to the obtained results, the dust export from N. Africa, which occurs under the prevalence of a trough over the western MB, and a ridge over the central MB, extends from southwest to northeast along two axes, one in the western and another in the central Mediterranean, covering remote areas up to the coasts of southern Europe, including the Balearic and Tyrrhenian Seas, the Italian peninsula, the Ionian and Adriatic Seas, and the Balkan peninsula. The analysis provides evidence of the formation of mixed-phase clouds, with high cloud-top heights (CTH higher than 10 km) and low cloud-top temperatures (CTT as low as 230 K), which spatiotemporally coincide with the high dust loadings that provide the necessary CCN and IN. Dust aerosols are transported either in the boundary layer (within the first 1–2 km) of areas close to the North African dust source areas or in the free troposphere over the Mediterranean Sea and the Italian and Balkan peninsulas (between 2 and 8 km). Distinct and extended layers of remarkable temperature inversions (up to 20 K/km) are created below the exported dust layers in the boundary layer of Mediterranean Sea areas, while weak/reduced lapse rates are formed over continental areas of MB undergoing the dust transport. Such modifications of temperature fields are important for the dynamics of the atmosphere of MB.