New cloud property datasets based on measurements from the passive imaging satellite sensors AVHRR, MODIS, ATSR2, AATSR and MERIS are presented. Two retrieval systems were developed that include components for cloud detection and cloud typing followed by cloud property retrievals based on the optimal estimation (OE) technique. The OE-based retrievals are applied to simultaneously retrieve cloud-top pressure, cloud particle effective radius and cloud optical thickness using measurements at visible, near-infrared and thermal infrared wavelengths, which ensures spectral consistency. The retrieved cloud properties are further processed to derive cloud-top height, cloud-top temperature, cloud liquid water path, cloud ice water path and spectral cloud albedo. The Cloud_cci products are pixel-based retrievals, daily composites of those on a global equal-angle latitude–longitude grid, and monthly cloud properties such as averages, standard deviations and histograms, also on a global grid. All products include rigorous propagation of the retrieval and sampling uncertainties. Grouping the orbital properties of the sensor families, six datasets have been defined, which are named AVHRR-AM, AVHRR-PM, MODIS-Terra, MODIS-Aqua, ATSR2-AATSR and MERIS+AATSR, each comprising a specific subset of all available sensors. The individual characteristics of the datasets are presented together with a summary of the retrieval systems and measurement records on which the dataset generation were based. Example validation results are given, based on comparisons to well-established reference observations, which demonstrate the good quality of the data. In particular the ensured spectral consistency and the rigorous uncertainty propagation through all processing levels can be considered as new features of the Cloud_cci datasets compared to existing datasets. In addition, the consistency among the individual datasets allows for a potential combination of them as well as facilitates studies on the impact of temporal sampling and spatial resolution on cloud climatologies.For each dataset a digital object identifier has been issued:Cloud_cci AVHRR-AM: https://doi.org/10.5676/DWD/ESA_Cloud_cci/AVHRR-AM/V002Cloud_cci AVHRR-PM: https://doi.org/10.5676/DWD/ESA_Cloud_cci/AVHRR-PM/V002Cloud_cci MODIS-Terra: https://doi.org/10.5676/DWD/ESA_Cloud_cci/MODIS-Terra/V002Cloud_cci MODIS-Aqua: https://doi.org/10.5676/DWD/ESA_Cloud_cci/MODIS-Aqua/V002Cloud_cci ATSR2-AATSR: https://doi.org/10.5676/DWD/ESA_Cloud_cci/ATSR2-AATSR/V002Cloud_cci MERIS+AATSR: https://doi.org/10.5676/DWD/ESA_Cloud_cci/MERIS+AATSR/V002

Clouds and aerosols contribute the largest uncertainty to current estimates and interpretations of the Earth’s changing energy budget. Here we use a new-generation large-domain large-eddy model, ICON-LEM (ICOsahedral Non-hydrostatic Large Eddy Model), to simulate the response of clouds to realistic anthropogenic perturbations in aerosols serving as cloud condensation nuclei (CCN). The novelty compared to previous studies is that (i) the LEM is run in weather prediction mode and with fully interactive land surface over a large domain and (ii) a large range of data from various sources are used for the detection and attribution. The aerosol perturbation was chosen as peak-aerosol conditions over Europe in 1985, with more than fivefold more sulfate than in 2013. Observational data from various satellite and ground-based remote sensing instruments are used, aiming at the detection and attribution of this response. The simulation was run for a selected day (2 May 2013) in which a large variety of cloud regimes was present over the selected domain of central Europe. It is first demonstrated that the aerosol fields used in the model are consistent with corresponding satellite aerosol optical depth retrievals for both 1985 (perturbed) and 2013 (reference) conditions. In comparison to retrievals from ground-based lidar for 2013, CCN profiles for the reference conditions were consistent with the observations, while the ones for the 1985 conditions were not. Similarly, the detection and attribution process was successful for droplet number concentrations: the ones simulated for the 2013 conditions were consistent with satellite as well as new ground-based lidar retrievals, while the ones for the 1985 conditions were outside the observational range. For other cloud quantities, including cloud fraction, liquid water path, cloud base altitude and cloud lifetime, the aerosol response was small compared to their natural variability. Also, large uncertainties in satellite and ground-based observations make the detection and attribution difficult for these quantities. An exception to this is the fact that at a large liquid water path value (LWP > 200 g m⁻²), the control simulation matches the observations, while the perturbed one shows an LWP which is too large. The model simulations allowed for quantifying the radiative forcing due to aerosol–cloud interactions, as well as the adjustments to this forcing. The latter were small compared to the variability and showed overall a small positive radiative effect. The overall effective radiative forcing (ERF) due to aerosol–cloud interactions (ERFaci) in the simulation was dominated thus by the Twomey effect and yielded for this day, region and aerosol perturbation −2.6 W m⁻². Using general circulation models to scale this to a global-mean present-day vs. pre-industrial ERFaci yields a global ERFaci of −0.8 W m⁻².

A new retrieval of total column water vapour (TCWV) from daytime measurements over land of the Ocean and Land Colour Instrument (OLCI) on-board the Copernicus Sentinel-3 missions is presented. The Copernicus Sentinel-3 OLCI Water Vapour product (COWa) retrieval algorithm is based on the differential absorption technique, relating TCWV to the radiance ratio of non-absorbing band and nearby water vapour absorbing band and was previously also successfully applied to other passive imagers Medium Resolution Imaging Spectrometer (MERIS) and Moderate Resolution Imaging Spectroradiometer (MODIS). One of the main advantages of the OLCI instrument regarding improved TCWV retrievals lies in the use of more than one absorbing band. Furthermore, the COWa retrieval algorithm is based on the full Optimal Estimation (OE) method, providing pixel-based uncertainty estimates, and transferable to other Near-Infrared (NIR) based TCWV observations. Three independent global TCWV data sets, i.e., Aerosol Robotic Network (AERONET), Atmospheric Radiation Measurement (ARM) and U.S. SuomiNet, and a German Global Navigation Satellite System (GNSS) TCWV data set, all obtained from ground-based observations, serve as reference data sets for the validation. Comparisons show an overall good agreement, with absolute biases between 0.07 and 1.31 kg/m² and root mean square errors (RMSE) between 1.35 and 3.26 kg/m². This is a clear improvement in comparison to the operational OLCI TCWV Level 2 product, for which the bias and RMSEs range between 1.10 and 2.55 kg/m² and 2.08 and 3.70 kg/m², respectively. A first evaluation of pixel-based uncertainties indicates good estimated uncertainties for lower retrieval errors, while the uncertainties seem to be overestimated for higher retrieval errors.

This study presents the first analysis of small‐scale convective structures observed in a total column water vapor (TCWV) field obtained from full‐resolution Medium Resolution Imaging Spectrometer (MERIS) near‐infrared measurements. The high‐resolution MERIS TCWV field for a high‐pressure event occurring in May over central Europe allows the detection of horizontal convective rolls, due to the observation of parallel bands of alternating low‐ and high‐TCWV values. The bands are aligned parallel to the boundary layer winds obtained from a numerical weather prediction model and radiosonde data. Closer examination further reveals that cloud streets observed in the east extend along bands of maximum TCWV. From a quantitative analysis of the TCWV data, combined with auxiliary data, it is shown that the roll wavelength and aspect ratio can be determined, which are found to be 6.5 km and 4.2, respectively, for this case study.

Water vapor concentration structures in the atmosphere are well approximated horizontally by Gaussian random fields at small scales (≲6 km). These Gaussian random fields have a spatial correlation in accordance with a structure function with a two-thirds slope, following the corresponding law from Kolmogorov's theory of turbulence. This is proven by showing that the horizontal structure functions measured by several satellite instruments and radiosonde measurements do indeed follow the two-thirds law. High-spatial-resolution retrievals of total column water vapor (TCWV) obtained from the Ocean and Land Color Instrument (OLCI) on board the Sentinel-3 series of satellites also qualitatively show a Gaussian random field structure. As a consequence, the atmosphere has an inherently stochastic component associated with the horizontal small-scale water vapor features, which, in turn, can make deterministic forecasting or nowcasting difficult. These results can be useful in areas where high-resolution modeling of water vapor is required, such as the estimation of the water vapor variance within a region or when searching for consistency between different water vapor measurements in neighboring locations. In terms of weather forecasting or nowcasting, the water vapor horizontal variability could be important in estimating the uncertainty of the atmospheric processes driving convection.

Complex terrain features—in particular, environmental conditions, high population density and potential socio-economic damage—make the Trans-Mexican Volcanic Belt (TMVB) of particular interest regarding the study of deep convection and related severe weather. In this research, 10 years of Moderate-Resolution Imaging Spectroradiometer (MODIS) cloud observations are combined with Climate Hazards Group Infrared Precipitation with Station (CHIRPS) rainfall data to characterize the spatio-temporal distribution of deep convective clouds (DCCs) and their relationship to extreme precipitation. From monthly distributions, wet and dry phases are identified for cloud fraction, deep convective cloud frequency and convective precipitation. For both DCC and extreme precipitation events, the highest frequencies align just over the higher elevations of the TMVB. A clear relationship between DCCs and terrain features, indicating the important role of orography in the development of convective systems, is noticed. For three sub-regions, the observed distributions of deep convective cloud and extreme precipitation events are assessed in more detail. Each sub-region exhibits different local conditions, including terrain features, and are known to be influenced differently by emerging moisture fluxes from the Gulf of Mexico and the Pacific Ocean. The observed distinct spatio-temporal variabilities provide the first insights into the physical processes that control the convective development in the study area. A signal of the midsummer drought in Mexico (i.e., “canícula”) is recognized using MODIS monthly mean cloud observations.