Both dc and ac magnetic susceptibility have been carefully measured and analyzed in order to determine the features of the low-temperature magnetic state of the highly frustrated compound. The scaling analysis of the nonlinear part of the dc magnetic susceptibility gives clues that indicate that the nature of the magnetic state below does not correspond to a conventional spin glass. This idea is further confirmed by the study of the dynamic scaling that also differs from what is expected for a conventional spin glass. A progressive change towards a more conventional magnetic ordering below is observed by substituting Ga atoms by Fe atoms in the compound . For x=1.5, both the scaling analysis of the nonlinear part of the dc magnetic susceptibility and the dynamic scaling seem to indicate that a true spin-glass phase transition does exist at . This change in the magnetic behavior is attributed to the fact that the presence of a magnetic atom in the 4 sites as a first neighbor of the Cr atoms, located in the 12k sites, will impose a ‘‘local preferential direction’’ for the magnetic moments removing somehow the strong intrinsic magnetic frustration of the kagomé lattice.
16 January 2019 in Theoretical and Applied Climatology