Nonwovens made of recycled carbon fibers (rCF) and thermoplastic (TP) fibers have excellent economic and ecological potential. In contrast to new fibers, recycled carbon fibers are significantly cheaper, and the CO₂ footprint is mostly compensated by energy savings in the first product life cycle. The next step for this promising material is its industrial serial use. Therefore, we analyzed the process chain from fiber to composite material. Initially, the rCF length at different positions during the carding process was measured. Thereafter, we evaluated the influence of the TP fibers on the processing, fiber shortening, and mechanical properties. Finally, several nonwovens with different TP fibers and fiber volume contents between 15 vol% and 30 vol% were produced, consolidated by hot-pressing, and tested by four-point bending to determine the mechanical values. The fiber length reduction ranged from 20.6% to 28.4%. TP fibers cushioned the rCF against mechanical stress but held rCF fragments back due to their crimp. The resulting bending strength varied from 301 to 405 MPa, and the stiffness ranged from 16.3 to 30.1 GPa. Design recommendations for reduced fiber shortening are derived as well as material mixtures that offer better homogeneity and higher mechanical properties.

This study focuses on producing and processing highly aligned tapes from recycled carbon fibers (rCFs). The rCFs are processed with a modified carding machine, oriented through a specialized subsequent process and consolidated into a semi-finished product. These rCF-tapes are placed onto a two-dimensional tool using an adapted automated fiber placement (AFP) technology to demonstrate a novel approach of producing composites from highly oriented recycled materials. The semi-finished stacks are consolidated in a heating press and test coupons are tested according to corresponding standards. The rCF-tapes are evaluated using methods such as tensile and flexural testing and determination of fiber volume content. Mechanical values are assessed by processing various generations of rCF-tapes and comparing them to each other and to virgin fiber tapes (vCF-tapes) made of the same type of carbon fiber and matrix. Microscopic imaging is also performed to analyze the quality of the resulting composites. In this study, a tensile strength of up to 1100 MPa in the fiber direction and stiffness of up to 80 GPa at a fiber volume content (FVC) of approximately 40% were achieved. The results highlight the strong potential and benefits of using highly oriented rCF-tapes and demonstrate the suitability of fiber placement technologies for those recycled materials.