Co ultrathin films, of various thicknesses (0.8 nm ⩽ t _Co ⩽ 2.5 nm), have been grown by sputtering on Si substrates, using Pt buffer layers and different capping layers (Cu, Ir, MgO and Pt). The x-ray diffraction revealed that our films have a (1 1 1) out-of-plane texture with various degrees of strains. Their magnetic properties have been studied by vibrating sample magnetometry (VSM) and Brillouin light scattering (BLS) in the Damon–Eshbach geometry. VSM characterizations revealed that films with Co thickness below (above) the spin reorientation transition thickness, which is capping layer dependent, are perpendicularly (in-plane) magnetized, suggesting the existence of an interface anisotropy. The surface anisotropy constant was found to be 1.42 ± 0.02 erg cm ⁻² and of 1.33 ± 0.02 erg cm ⁻² for the Pt/Co/Cu and Pt/Co/Ir samples, respectively, suggesting that it is due to the Pt/Co interface and that the top Co/Cu, Co/Pt or Co/Ir interfaces have a minor contribution. A lower value of 1.07 ± 0.02 erg cm ⁻² has been obtained for Pt/Co/MgO most probably due to over-oxidation of Co at the Co/MgO interface. The BLS measurements revealed a pronounced nonreciprocal spin waves propagation, due to the interfacial Dzyaloshinskii–Moriya interaction (iDMI) induced by Pt interface with Co, which increases with decreasing Co thickness. The magnetic dead layer has been taken into account to precisely determine the surface iDMI constant D _s estimated at −0.8 pJ m ⁻¹ , −1.05 pJ m ⁻¹ and −0.95 pJ m ⁻¹ , respectively for Pt/Co/Ir, Pt/Co/Cu and Pt/Co/MgO for sample thicknesses where a linear thickness dependence of the effective iDMI constant has been observed.

Perpendicular magnetic anisotropy (PMA) in ultrathin magnetic structures is a key ingredient for the development of electrically controlled spintronic devices. Due to their relatively large spin polarization, high Curie temperature, and low Gilbert damping, the Co-based full Heusler alloys are of special importance from a scientific and applications point of view. Here, we study the mechanisms responsible for the PMA in Pt/Co-based full Heusler alloy/MgO thin-film structures. We show that the ultrathin Heusler films exhibit strong PMA even in the absence of magnetic annealing. By means of ferromagnetic resonance experiments, we demonstrate that the effective magnetization shows a two-regime behavior depending on the thickness of the Heusler layers. Using Auger spectroscopy measurements, we evidence interdiffusion at the underlayer/Heusler interface and the formation of an interfacial CoFe-rich layer which causes the two-regime behavior. In the case of the ultrathin films, the interfacial CoFe-rich layer promotes the strong PMA through the electronic hybridization of the metal alloy and oxygen orbitals across the ferromagnet/MgO interface. In addition, the interfacial CoFe-rich layer is also generating an increase of the Gilbert damping for the ultrathin films beyond the spin-pumping effect. Our results illustrate that the strong PMA is not an intrinsic property of the Heusler/MgO interface but it is actively influenced by the interdiffusion, which can be tuned by a proper choice of the underlayer material, as we show for the cases of the Pt, Ta, and Cr underlayers.

Magnetization switching by current induced spin–orbit torques (SOTs) in heavy metal/ferromagnetic metal/oxide structures is of great research interest due to its potential applications in the field of low power consumption spintronic devices. Here, we study the Slonczewski-like and the field-like SOT effective fields in β-W/Co₂FeAl/MgO structures showing perpendicular magnetic anisotropy (PMA). We characterize the SOT effective fields using harmonic Hall voltage measurements and we point out the essential role of the planar Hall effect corrections. We estimate that for bulk β-W an effective spin Hall angle as large as 0.3 ± 0.03 and a spin diffusion length of 2.2 ± 0.3 nm. Moreover, we demonstrate SOT-induced magnetization switching for charge current densities of the order of 10⁶ A cm⁻².

The occurrence of both interlayer exchange coupling and perpendicular magnetic anisotropy is evidenced in Pt/Co/Ir/Co/Pt magnetron sputtered structures. We point out the effect of lattice strains on stabilizing the perpendicular magnetic anisotropy. The surface magnetic anisotropy constant is around 1.76 erg cm ⁻² and around 1.5 erg cm ⁻² for the Co layers, depending on their positioning within the stack. We demonstrate a relatively high interlayer exchange constant of −2.5 erg cm ⁻² at the first antiferromagnetic coupling maximum corresponding to an exchange field larger than 12 kOe. The interlayer exchange coupling shows remarkable annealing endurance being preserved for annealing temperatures up to 400 °C.