Quasi‐phase matching (QPM) is a technique in nonlinear optics for achieving efficient energy exchange among optical waves at different frequencies, by spatially modulating the quadratic nonlinearity (χ ⁽²⁾) of the medium. To realize the full potential of QPM, 3D spatial modulation of χ ⁽²⁾ is required. This has become experimentally feasible recently thanks to the invention of femtosecond laser‐based nonlinearity engineering in ferroelectric crystals. Herein, the first experimental demonstration of QPM second harmonic generation (SHG) in a nonlinear cubic crystal system is presented, in which χ ⁽²⁾ modulations form simple cubic, body‐centered cubic, face‐centered cubic, and diamond cubic lattices, respectively. The experimental results indicate that these nonlinear cubic structures share the same primary reciprocal lattice vectors (RLVs), but possess different Fourier coefficients (in conventional cells), leading to SHG with similar angular resonances but various intensity distributions in the far field. This work contributes to a comprehensive understanding of nonlinear optical processes in 3D periodic media, and thus sheds light on the development of high‐performance QPM devices.

Ferroelectric domain engineering has wide applications in optical and electronic industries. Compared with traditional electric field poling, femtosecond laser poling has many advantages, such as higher fabrication resolution, 3D engineering applicability, and lower costs of production. In this review, the recent research progress on ferroelectric domain engineering with femtosecond laser pulses is presented. We show the latest results, including complex domain structures fabricated in various kinds of ferroelectric crystals, and discuss the influence of laser poling parameters and conditions on the morphologies of inverted domains and their physical mechanisms. The technical challenges to overcome in future are also briefly discussed.

A novel 2H-phase transition metal dichalcogenide (TMD)–tantalum selenide (TaSe₂) with metallic bandgap structure is a potential photoelectric material. A band structure simulation of TaSe₂ via ab initio method indicated its metallic property. An effective multilayered TaSe₂ saturable absorber (SA) was fabricated using liquid-phase exfoliation and optically driven deposition. The prepared 2H–TaSe₂ SA was successfully used for a dual-wavelength Q-switched fiber laser with the minimum pulse width of 2.95 μs and the maximum peak power of 64 W. The repetition rate of the maximum pulse energy of 89.9 kHz was at the level of 188.9 nJ. The metallic 2H–TaSe₂ with satisfactory saturable absorbing capability is a promising candidate for pulsed laser applications.

Nonlinear photonic crystals with 3D orthorhombic lattice structures were fabricated using the femtosecond laser-poling technique in ferroelectric Sr_0.28Ba_0.72Nb₂O₆ (SBN) crystals. The crystals were used to demonstrate the possibility of generating cascaded third-harmonic waves in optically poled ferroelectric structures. The spectral response and conversion efficiency of the third-harmonic process were experimentally investigated. While the nonlinear cascading processes can be commonly realized in electric-field-poled ferroelectric crystals, their generation in optically poled ferroelectric domain structures have not been reported elsewhere. In addition to the fully phase-matched nonlinear interaction, Cherenkov-type third-harmonic generation that fulfills the longitudinal phase-matching condition was also experimentally studied. Our study contributes to exploring the full potential of optically induced nonlinear photonic crystals and provides a new choice of materials for third-harmonic generation.

This paper demonstrates the sorting and detection of near-infrared vortex light using a nonlinear Dammann vortex grating. By incorporating a forked structure into the nonlinear Dammann grating, the resulting nonlinear Dammann vortex grating is capable of converting near-infrared Gaussian light into a visible vortex array. The array comprises 49 independent detection channels, each of which can precisely control the inherent topological charge values. When the topological charge value of a detection channel’s vortex light matches that of the incident vortex, the vortex degenerates into a Gaussian spot, thereby enabling the detection of the incident vortex’s topological charge. Our experimental results show that this grating, with its 49 independent detection channels, can detect the topological charge values of vortex light in the near-infrared range from l = −12 to +12 in real-time. Compared to existing solutions, this grating offers enhanced versatility and has potential applications in optical communication systems for the transmission, reception, and multiplexing of OV beams.

We present the development of an As ₂ S ₃ fiber-based reusable inline optical connector; and, for the first time to the best of our knowledge, integrated it into a 2 μm chirped pulse amplification system as the pulse stretcher. By this mechanism, a near 20 times pulse stretching ratio was achieved in 0.5 m-long this As ₂ S ₃ fiber and the introduction of insertion loss as low as 2.84 dB while it was connected with silica fiber. After the follow-up fiber amplification and self-compression mechanism, the laser average output power was boosted to 1.97 W and pulse duration was optimized to 2.53 ps. Moreover, to further inspect the laser pulse property, the pulses were then delivered into a 5.3 m-long ZrF ₄ -BaF ₂ -LaF ₃ -AlF ₃ -NaF (ZBLAN) fiber which was fusion spliced to SM1950 fiber. Thanks to the 0.4-dB low fusion splice loss between these fibers, a 1.56-W supercontinuum source with bandwidth of 1.93-3.50 μm is obtained. The measured two hours of root-mean-square value of power fluctuation of this laser source is 0.13%, indicating an ultra-high long-term power stability. This work will lay a solid foundation in the realization of the all-fiber structured high-power thulium-doped fiber amplifier with high compactness.