The eXawatt Center for Extreme Light Studies project aimed to create a large scientific infrastructure based on lasers with giant peak power. The project relies on the significant progress achieved in the last decade. The planned infrastructure will incorporate a unique light source with a pulse power of 600 PW using optical parametric chirped pulse amplification in large-aperture KD₂PO₄, deuterated potassium dihydrogen phosphate crystals. The interaction of such laser radiation with matter represents a completely new fundamental physics. The direct study of the space–time structure of vacuums and other unknown phenomena at the frontier of high-energy physics and the physics of superstrong fields will be challenged. Expected applications will include the development of compact particle accelerators, the generation of ultrashort pulses of hard X-ray and gamma radiation for material science enabling one to probe material samples with unprecedented spatial and temporal resolution, the development of new radiation and particle sources, etc. The paper is translation from Russian [Kvantovaya Elektronika 53, 95 (2023)].

The PEARL laser output pulse with a duration of 60-70 fs was compressed to 11 fs after passing through a 5-mm thick silica plate and reflecting from two chirping mirrors with a total dispersion of -250 fs². The experiments were carried out for the B-integral values up to 19 without damage of the optical elements, which indicates that small-scale self-focusing was suppressed. The results obtained show the possibility of further nonlinear compression scaling to multipetawatt power in pulses with duration commensurate with the field period.

The pulse spectrum at the laser output was broadened due to self-phase modulation in fused silica and then the pulse was compressed by chirped mirrors. It was demonstrated that with an optimal choice of mirror dispersion a pulse with an energy of 17 J can be compressed from 70 to 14 fs. This compression after compressor approach has undoubted merits: simplicity, low cost, negligible pulse energy losses, and applicability to any high-power laser.

All space–time coupling effects arising in an asymmetric optical compressor consisting of two non-identical pairs of diffraction gratings are described analytically. In each pair, the gratings are identical and parallel to each other, whereas the distance between the gratings, the groove density and the angle of incidence are different in different pairs. It is shown that the compressor asymmetry does not affect the far-field fluence and on-axis focal intensity. The main distinctive feature of the asymmetric compressor is spatial noise lagging behind or overtaking the main pulse in proportion to the transverse wave vector. This results in a degraded contrast but reduces beam fluence fluctuations at the compressor output. Exact expressions are obtained for the spectrum of fluence fluctuations and fluence root mean square that depends only on one parameter characterizing compressor asymmetry. The efficiency of small-scale self-focusing suppression at subsequent pulse post-compression is estimated.

The input pulse of the laser PEARL with energy of 18 J and pulse duration of about 60 fs was compressed to 10 fs after passage through a 4-mm-thick KDP crystal and reflection at two chirped mirrors with sum dispersion of −200 fs². The experiments were performed for the В-integral values from 5 to 19 without visible damage to the optical elements, which indicates that small-scale self-focusing is not a significant issue. It was shown that, by virtue of the low dispersion of the group velocity, the KDP crystal has some advantages over silica: a larger pulse compression coefficient, especially at a small value of the В-integral (B = 5, …, 9), lower absolute values of chirped mirror dispersion, and also a possibility to control the magnitude of nonlinearity and dispersion by changing crystal orientation.

By extending the concept of thin film compression [Mourou et al., Eur. Phys. J. Spec. Top. 223(6), 1181 (2014)] to a thin plate, nonlinear post-compression from 24 fs to 13 fs of sub-petawatt laser pulses is demonstrated experimentally using a 1 mm-thick silica plate and chirped mirrors with a total anomalous dispersion of −50 fs². The measurements were implemented with a specially designed dispersionless vacuum frequency-resolved optical gating, which is based on second harmonic generation of tested pulses in a 10 μm β-barium borate crystal glued on a 1 mm fused silica substrate. The used compression scheme is implemented in a geometry compatible with high power on-target experiment realization.